Effect of Ga doping on the catalytic performance of Zn-ZSM-5 for CO2-assisted oxidative dehydrogenation of C2H6 Article Swipe
Hongtao Wen
,
Xinru Han
,
Lina Zhang
,
Yongdong Chen
,
Wei Wei
,
Nannan Sun
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1016/j.jcou.2025.103066
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1016/j.jcou.2025.103066
Using a low silica-to-alumina ratio NaZSM-5 zeolite as the support, a bimetallic modified catalyst, GaxZnZ5, was prepared through ion-exchange method for CO2-mediated oxidative dehydrogenation of C2H6 (CO2-ODH). Based on systematic characterization and evaluation, it was found that Zn is the primary active component in the catalytic system for activating C2H6, but it is merely active towards CO2, leading to rapid catalyst deactivation. Under the influence of Ga species, CO2 can readily engage into the reaction network. During the initial stage of the reaction, the activated CO2 primarily participants in dry reforming with C2H6-x species that rapidly formed on highly active Zn sites. However, the rapid cleavage of C-H bonds on these Zn sites leads to significant carbon deposition and subsequent deactivation. Following this rapid deactivation phase, CO2 becomes involved in the reaction through the reverse water-gas shift (RWGS) reaction and carbon elimination reactions, thereby shifting the reaction equilibrium towards C2H4 formation while alleviating the accumulation of carbon deposition and thus enhancing stability. With the optimum catalyst (Ga0.27ZnZ5), excellent and stable performance with 22.64 % C2H4 yield and nearly 100 % selectivity could be achieved after an induction period of ca. 100 minutes, these are among the highest values reported so far.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.jcou.2025.103066
- OA Status
- gold
- Cited By
- 1
- References
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- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4408730870Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.jcou.2025.103066Digital Object Identifier
- Title
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Effect of Ga doping on the catalytic performance of Zn-ZSM-5 for CO2-assisted oxidative dehydrogenation of C2H6Work title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-03-22Full publication date if available
- Authors
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Hongtao Wen, Xinru Han, Lina Zhang, Yongdong Chen, Wei Wei, Nannan SunList of authors in order
- Landing page
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https://doi.org/10.1016/j.jcou.2025.103066Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://doi.org/10.1016/j.jcou.2025.103066Direct OA link when available
- Concepts
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Dehydrogenation, ZSM-5, Oxidative phosphorylation, Catalysis, Doping, Materials science, Chemical engineering, Chemistry, Organic chemistry, Zeolite, Optoelectronics, Engineering, BiochemistryTop concepts (fields/topics) attached by OpenAlex
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1Total citation count in OpenAlex
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2025: 1Per-year citation counts (last 5 years)
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32Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.with | 91, 171 |
| abstract_inverted_index.22.64 | 172 |
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| abstract_inverted_index.C2H6, | 49 |
| abstract_inverted_index.Under | 62 |
| abstract_inverted_index.Using | 0 |
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| abstract_inverted_index.among | 194 |
| abstract_inverted_index.bonds | 108 |
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| abstract_inverted_index.yield | 175 |
| abstract_inverted_index.(RWGS) | 137 |
| abstract_inverted_index.C2H6-x | 92 |
| abstract_inverted_index.During | 76 |
| abstract_inverted_index.active | 41, 54, 99 |
| abstract_inverted_index.carbon | 116, 140, 156 |
| abstract_inverted_index.engage | 71 |
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| abstract_inverted_index.highly | 98 |
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| abstract_inverted_index.phase, | 125 |
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| abstract_inverted_index.system | 46 |
| abstract_inverted_index.values | 197 |
| abstract_inverted_index.NaZSM-5 | 5 |
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| abstract_inverted_index.highest | 196 |
| abstract_inverted_index.initial | 78 |
| abstract_inverted_index.leading | 57 |
| abstract_inverted_index.optimum | 164 |
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| abstract_inverted_index.readily | 70 |
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| abstract_inverted_index.through | 17, 132 |
| abstract_inverted_index.towards | 55, 148 |
| abstract_inverted_index.zeolite | 6 |
| abstract_inverted_index.GaxZnZ5, | 14 |
| abstract_inverted_index.However, | 102 |
| abstract_inverted_index.achieved | 183 |
| abstract_inverted_index.catalyst | 60, 165 |
| abstract_inverted_index.cleavage | 105 |
| abstract_inverted_index.involved | 128 |
| abstract_inverted_index.minutes, | 191 |
| abstract_inverted_index.modified | 12 |
| abstract_inverted_index.network. | 75 |
| abstract_inverted_index.prepared | 16 |
| abstract_inverted_index.reaction | 74, 131, 138, 146 |
| abstract_inverted_index.reported | 198 |
| abstract_inverted_index.shifting | 144 |
| abstract_inverted_index.species, | 67 |
| abstract_inverted_index.support, | 9 |
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| abstract_inverted_index.activated | 84 |
| abstract_inverted_index.catalyst, | 13 |
| abstract_inverted_index.catalytic | 45 |
| abstract_inverted_index.component | 42 |
| abstract_inverted_index.enhancing | 160 |
| abstract_inverted_index.excellent | 167 |
| abstract_inverted_index.formation | 150 |
| abstract_inverted_index.induction | 186 |
| abstract_inverted_index.influence | 64 |
| abstract_inverted_index.oxidative | 22 |
| abstract_inverted_index.primarily | 86 |
| abstract_inverted_index.reaction, | 82 |
| abstract_inverted_index.reforming | 90 |
| abstract_inverted_index.water-gas | 135 |
| abstract_inverted_index.(CO2-ODH). | 26 |
| abstract_inverted_index.activating | 48 |
| abstract_inverted_index.bimetallic | 11 |
| abstract_inverted_index.deposition | 117, 157 |
| abstract_inverted_index.reactions, | 142 |
| abstract_inverted_index.stability. | 161 |
| abstract_inverted_index.subsequent | 119 |
| abstract_inverted_index.systematic | 29 |
| abstract_inverted_index.alleviating | 152 |
| abstract_inverted_index.elimination | 141 |
| abstract_inverted_index.equilibrium | 147 |
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| abstract_inverted_index.selectivity | 180 |
| abstract_inverted_index.significant | 115 |
| abstract_inverted_index.CO2-mediated | 21 |
| abstract_inverted_index.accumulation | 154 |
| abstract_inverted_index.deactivation | 124 |
| abstract_inverted_index.ion-exchange | 18 |
| abstract_inverted_index.participants | 87 |
| abstract_inverted_index.(Ga0.27ZnZ5), | 166 |
| abstract_inverted_index.deactivation. | 61, 120 |
| abstract_inverted_index.dehydrogenation | 23 |
| abstract_inverted_index.characterization | 30 |
| abstract_inverted_index.silica-to-alumina | 3 |
| cited_by_percentile_year.max | 95 |
| cited_by_percentile_year.min | 91 |
| countries_distinct_count | 0 |
| institutions_distinct_count | 6 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/6 |
| sustainable_development_goals[0].score | 0.5600000023841858 |
| sustainable_development_goals[0].display_name | Clean water and sanitation |
| citation_normalized_percentile.value | 0.65551012 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |