Effect of Steam on Carbonation of CaO in Ca-Looping Article Swipe
Ruzhan Bai
,
Na Li
,
Quansheng Liu
,
Shenna Chen
,
Qi Liu
,
Xing Zhou
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.3390/molecules28134910
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.3390/molecules28134910
Ca-looping is an effective way to capture CO2 from coal-fired power plants. However, there are still issues that require further study. One of these issues is the effect of steam on the Ca-looping process. In this paper, a self-madethermogravimetric analyzer that can achieve rapid heating and cooling is used to measure the change of sample weight under constant temperature conditions. The parameters of the Ca-looping are studied in detail, including the addition of water vapor alone in the calcination or carbonation stage and the calcination/carbonation reaction temperatures for both calcination and carbonation stages with water vapor. Steam has a positive overall effect on CO2 capture in the Ca-looping process. When steam is present in both calcination and carbonation processes, it increases the decomposition rate of CaCO3 and enhances the subsequent carbonation conversion of CaO. However, when steam was present only in the calcination process, there was lower CaO carbonation conversion in the following carbonation process. In contrast, when steam was present in the carbonation stage, CO2 capture was improved. Sample characterizations after the reaction showed that although water vapor had a negative effect on the pore structure, adding water vapor increased the diffusion coefficient of CO2 and the carbonation conversion rate of CaO.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/molecules28134910
- https://www.mdpi.com/1420-3049/28/13/4910/pdf?version=1687422277
- OA Status
- gold
- Cited By
- 11
- References
- 37
- Related Works
- 10
- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4381804572Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/molecules28134910Digital Object Identifier
- Title
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Effect of Steam on Carbonation of CaO in Ca-LoopingWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-06-22Full publication date if available
- Authors
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Ruzhan Bai, Na Li, Quansheng Liu, Shenna Chen, Qi Liu, Xing ZhouList of authors in order
- Landing page
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https://doi.org/10.3390/molecules28134910Publisher landing page
- PDF URL
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https://www.mdpi.com/1420-3049/28/13/4910/pdf?version=1687422277Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
- OA URL
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https://www.mdpi.com/1420-3049/28/13/4910/pdf?version=1687422277Direct OA link when available
- Concepts
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Carbonation, Calcination, Water vapor, Chemistry, Chemical engineering, Calcium looping, Materials science, Mineralogy, Catalysis, Organic chemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
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11Total citation count in OpenAlex
- Citations by year (recent)
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2025: 5, 2024: 5, 2023: 1Per-year citation counts (last 5 years)
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37Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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