Effects of crosslink density in zwitterionic hydrogel coatings on their antifouling performance and susceptibility to silt uptake Article Swipe
Julian Koc
,
Eric Schönemann
,
Robin Wanka
,
Nick Aldred
,
Anthony S. Clare
,
Harrison Gardner
,
Geoffrey Swain
,
Kelli Z. Hunsucker
,
André Laschewsky
,
Axel Rosenhahn
·
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1080/08927014.2020.1796983
YOU?
·
· 2020
· Open Access
·
· DOI: https://doi.org/10.1080/08927014.2020.1796983
Hydrogel coatings effectively reduce the attachment of proteins and organisms in laboratory assays, in particular when made from zwitterionic monomers. In field experiments with multiple species and non-living material, such coatings suffer from adsorption of particulate matter. In this study, the zwitterionic monomer 3-[N-(2-methacryloyloxyethyl)-N,N-dimethylammonio] propanesulfonate (SPE) was copolymerized with increasing amounts of the photo-crosslinker benzophenon-4-yloxyethyl methacrylate (BPEMA) to systematically alter the density of crosslinks between the polymer chains. The effect of increasing crosslink density on the antifouling (AF) performance of the coatings was investigated in laboratory assays and fields tests. In both cases, the AF performance was improved by increasing the crosslinker content. The coatings reduced protein, diatom, and barnacle accumulation, and showed better resistance to biomass accumulation. The findings underline that the marine AF performance of hydrogel coatings does not only depend on the specific chemical structure of the polymers, but also on their physico-chemical properties such as rigidity and swelling.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1080/08927014.2020.1796983
- OA Status
- green
- Cited By
- 33
- References
- 64
- Related Works
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- OpenAlex ID
- https://openalex.org/W3044576689
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W3044576689Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1080/08927014.2020.1796983Digital Object Identifier
- Title
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Effects of crosslink density in zwitterionic hydrogel coatings on their antifouling performance and susceptibility to silt uptakeWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2020Year of publication
- Publication date
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2020-07-02Full publication date if available
- Authors
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Julian Koc, Eric Schönemann, Robin Wanka, Nick Aldred, Anthony S. Clare, Harrison Gardner, Geoffrey Swain, Kelli Z. Hunsucker, André Laschewsky, Axel RosenhahnList of authors in order
- Landing page
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https://doi.org/10.1080/08927014.2020.1796983Publisher landing page
- Open access
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://figshare.com/articles/journal_contribution/Effects_of_crosslink_density_in_zwitterionic_hydrogel_coatings_on_their_antifouling_performance_and_susceptibility_to_silt_uptake/12848639Direct OA link when available
- Concepts
-
Biofouling, Methacrylate, Monomer, Chemical engineering, Polymer, Materials science, Swelling, Diatom, Adsorption, Polymer chemistry, Chemistry, Organic chemistry, Composite material, Biochemistry, Botany, Membrane, Engineering, BiologyTop concepts (fields/topics) attached by OpenAlex
- Cited by
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33Total citation count in OpenAlex
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2025: 7, 2024: 9, 2023: 3, 2022: 8, 2021: 5Per-year citation counts (last 5 years)
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64Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.polymer | 66 |
| abstract_inverted_index.reduced | 105 |
| abstract_inverted_index.species | 25 |
| abstract_inverted_index.Hydrogel | 0 |
| abstract_inverted_index.barnacle | 109 |
| abstract_inverted_index.chemical | 136 |
| abstract_inverted_index.coatings | 1, 30, 81, 104, 128 |
| abstract_inverted_index.content. | 102 |
| abstract_inverted_index.findings | 119 |
| abstract_inverted_index.hydrogel | 127 |
| abstract_inverted_index.improved | 97 |
| abstract_inverted_index.multiple | 24 |
| abstract_inverted_index.protein, | 106 |
| abstract_inverted_index.proteins | 7 |
| abstract_inverted_index.rigidity | 149 |
| abstract_inverted_index.specific | 135 |
| abstract_inverted_index.crosslink | 72 |
| abstract_inverted_index.material, | 28 |
| abstract_inverted_index.monomers. | 19 |
| abstract_inverted_index.organisms | 9 |
| abstract_inverted_index.polymers, | 140 |
| abstract_inverted_index.structure | 137 |
| abstract_inverted_index.swelling. | 151 |
| abstract_inverted_index.underline | 120 |
| abstract_inverted_index.adsorption | 33 |
| abstract_inverted_index.attachment | 5 |
| abstract_inverted_index.crosslinks | 63 |
| abstract_inverted_index.increasing | 49, 71, 99 |
| abstract_inverted_index.laboratory | 11, 85 |
| abstract_inverted_index.non-living | 27 |
| abstract_inverted_index.particular | 14 |
| abstract_inverted_index.properties | 146 |
| abstract_inverted_index.resistance | 114 |
| abstract_inverted_index.antifouling | 76 |
| abstract_inverted_index.crosslinker | 101 |
| abstract_inverted_index.effectively | 2 |
| abstract_inverted_index.experiments | 22 |
| abstract_inverted_index.particulate | 35 |
| abstract_inverted_index.performance | 78, 95, 125 |
| abstract_inverted_index.investigated | 83 |
| abstract_inverted_index.methacrylate | 55 |
| abstract_inverted_index.zwitterionic | 18, 41 |
| abstract_inverted_index.accumulation, | 110 |
| abstract_inverted_index.accumulation. | 117 |
| abstract_inverted_index.copolymerized | 47 |
| abstract_inverted_index.systematically | 58 |
| abstract_inverted_index.physico-chemical | 145 |
| abstract_inverted_index.propanesulfonate | 44 |
| abstract_inverted_index.photo-crosslinker | 53 |
| abstract_inverted_index.benzophenon-4-yloxyethyl | 54 |
| abstract_inverted_index.3-[<i>N</i>-(2-methacryloyloxyethyl)-<i>N</i>,<i>N-</i>dimethylammonio] | 43 |
| cited_by_percentile_year.max | 99 |
| cited_by_percentile_year.min | 89 |
| corresponding_author_ids | https://openalex.org/A5060772989, https://openalex.org/A5013726983 |
| countries_distinct_count | 3 |
| institutions_distinct_count | 10 |
| corresponding_institution_ids | https://openalex.org/I4210128116, https://openalex.org/I904495901 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/14 |
| sustainable_development_goals[0].score | 0.8899999856948853 |
| sustainable_development_goals[0].display_name | Life below water |
| citation_normalized_percentile.value | 0.90445356 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |