Efficient Free Charge Generation at Low-carrier Concentration in Chemically-doped Single-walled Carbon Nanotubes Article Swipe
Jeffrey L. Blackburn
,
Justin Earley
,
Obadiah G. Reid
,
Tucker L. Murrey
,
Evan A. Doud
,
Alexander M. Spokoyny
,
Martha Alejandra Hermosilla Palacios
,
Garry Rumbles
,
Andrew J. Ferguson
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-5054938/v1
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-5054938/v1
Free carrier generation in doped organic semiconductors is poorly understood, since assumed tight electron-hole binding conflicts with observed high free carrier yields. We experimentally investigate the roles of enthalpy, entropy, and local dielectric environment in free carrier generation and transport using isolated chemically doped semiconducting single-walled carbon nanotubes in low-dielectric solvent. Dopant chemical structure dramatically influences the observed changes in carrier density-dependent complex permittivity, with bulky dopants drastically increasing the local dielectric constant and electronic conductivity, even at carrier densities below one carrier per nanotube. The results are understood by considering the roles of entropic stabilization and a non-static dielectric constant, both of which lower the energy barrier for free charge generation. This understanding has important implications for designing doped organic systems and devices for enhanced carrier mobility, conductivity, and performance.
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.21203/rs.3.rs-5054938/v1
- https://www.researchsquare.com/article/rs-5054938/latest.pdf
- OA Status
- gold
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4403184432
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4403184432Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.21203/rs.3.rs-5054938/v1Digital Object Identifier
- Title
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Efficient Free Charge Generation at Low-carrier Concentration in Chemically-doped Single-walled Carbon NanotubesWork title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-10-08Full publication date if available
- Authors
-
Jeffrey L. Blackburn, Justin Earley, Obadiah G. Reid, Tucker L. Murrey, Evan A. Doud, Alexander M. Spokoyny, Martha Alejandra Hermosilla Palacios, Garry Rumbles, Andrew J. FergusonList of authors in order
- Landing page
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https://doi.org/10.21203/rs.3.rs-5054938/v1Publisher landing page
- PDF URL
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https://www.researchsquare.com/article/rs-5054938/latest.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
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https://www.researchsquare.com/article/rs-5054938/latest.pdfDirect OA link when available
- Concepts
-
Carbon nanotube, Doping, Free carrier, Charge (physics), Materials science, Charge carrier, Carbon fibers, Nanotechnology, Chemical engineering, Optoelectronics, Composite material, Physics, Composite number, Quantum mechanics, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
- Related works (count)
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10Other works algorithmically related by OpenAlex
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