Electric Charge Effect on the Water Mass Transfer across Mixed Aqueous–Organic Droplet Interfaces Article Swipe
Mercede Azizbaig Mohajer
,
Michael J. Gleichweit
,
Grégory David
,
Loren Ban
,
Felix Graber
,
Ruth Signorell
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1021/acs.jpca.5c06517
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1021/acs.jpca.5c06517
Understanding gas-particle mass transport is essential for predicting aerosol behavior in the atmosphere and in industrial processes. The mass accommodation coefficient, αM, is a key parameter describing this exchange. Defined as the probability of a gas-phase molecule adhering to a particle upon collision, αM presents a highly surface-sensitive property. Aqueous atmospheric aerosol droplets carry electric charges, which accumulate near the surface; however, their influence on the gas-particle mass transport remains elusive. To access the influence of charge on αM, we combined an aerosol charging method with photothermal single-particle spectroscopy, enabling direct water mass exchange measurements on the surface of single aerosol droplets. We investigated charged and neutral aqueous glycerol and tetraethylene glycol droplets across a wide range of concentrations and temperatures. The micrometre-sized droplets carried approximately 103 elementary charges─exceeding typical atmospheric aerosol charge levels─yet our results show that αM is independent of the droplet charge and instead is dominated by composition and temperature. Theoretical estimates of the charge-dipole and dipole-dipole interaction energies corroborate this finding, highlighting that under atmospherically relevant conditions, electric charge plays a negligible role in the mass accommodation process.
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- Landing Page
- https://doi.org/10.1021/acs.jpca.5c06517
- OA Status
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- References
- 39
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- https://openalex.org/W4415702279
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Electric Charge Effect on the Water Mass Transfer across Mixed Aqueous–Organic Droplet InterfacesWork title
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articleOpenAlex work type
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enPrimary language
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2025Year of publication
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2025-10-30Full publication date if available
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Mercede Azizbaig Mohajer, Michael J. Gleichweit, Grégory David, Loren Ban, Felix Graber, Ruth SignorellList of authors in order
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https://doi.org/10.1021/acs.jpca.5c06517Publisher landing page
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hybridOpen access status per OpenAlex
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| abstract_inverted_index.coefficient, | 20 |
| abstract_inverted_index.gas-particle | 1, 66 |
| abstract_inverted_index.highlighting | 165 |
| abstract_inverted_index.investigated | 103 |
| abstract_inverted_index.levels─yet | 133 |
| abstract_inverted_index.measurements | 94 |
| abstract_inverted_index.photothermal | 86 |
| abstract_inverted_index.temperature. | 152 |
| abstract_inverted_index.Understanding | 0 |
| abstract_inverted_index.accommodation | 19, 180 |
| abstract_inverted_index.approximately | 125 |
| abstract_inverted_index.charge-dipole | 157 |
| abstract_inverted_index.dipole-dipole | 159 |
| abstract_inverted_index.spectroscopy, | 88 |
| abstract_inverted_index.temperatures. | 120 |
| abstract_inverted_index.tetraethylene | 110 |
| abstract_inverted_index.10<sup>3</sup> | 126 |
| abstract_inverted_index.concentrations | 118 |
| abstract_inverted_index.α<sub>M</sub> | 43, 138 |
| abstract_inverted_index.atmospherically | 168 |
| abstract_inverted_index.single-particle | 87 |
| abstract_inverted_index.α<sub>M</sub>, | 21, 78 |
| abstract_inverted_index.micrometre-sized | 122 |
| abstract_inverted_index.surface-sensitive | 47 |
| abstract_inverted_index.charges─exceeding | 128 |
| cited_by_percentile_year | |
| corresponding_author_ids | https://openalex.org/A5059978764, https://openalex.org/A5084112820 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 6 |
| corresponding_institution_ids | https://openalex.org/I35440088 |
| citation_normalized_percentile |