Electrochemical Quartz Microbalance for Studying Electrodeposited Pt Catalysts for Methanol Oxidation Reaction Article Swipe
Bangfeng Zong
,
Xiao Jun Pan
,
Bo Wei
,
Lifang Zhang
,
Xiaoyan Feng
,
C. Hou
,
Hai Yan
,
Wenju Xie
,
Guicheng Liu
,
Ye Feng
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.3390/inorganics13040111
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.3390/inorganics13040111
Pt catalysts are investigated for methanol oxidation in direct methanol fuel cells, utilizing the electrochemical quartz microbalance method (EQCM) with exceptional resolution and sensitivity. Pt catalysts were deposited onto the gas-diffusion layer of carbon using stationary potential electrodeposition. Physical characterization and electrochemical tests were performed. SEM results showed that Pt presented dendrite crystals with nanoscale facets. Cyclic voltammetry (CV) demonstrated that the current density for the methanol oxidation reaction highly reached 1020 mA·cm−2 for the deposited Pt catalyst by EQCM. The dendrite crystal structures of deposited Pt provide much area for high catalytic activity. It found that the peak density of the Pt catalysts for the methanol oxidation reaction decreased after five cycles. Furthermore, the response frequency for the adsorption of the deposited Pt catalysts was investigated using EQCM and compared with commercial PtRu catalysts. The results showed that the response frequency of the Pt catalysts decreased more rapidly than that of the PtRu catalysts. It is possible for the adsorption of small organic molecules on Pt catalysts to occur during the methanol electro-oxidation with COad intermediates. The reaction mechanism is preliminarily discussed by the electrochemical measurement combined with EQCM.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/inorganics13040111
- https://www.mdpi.com/2304-6740/13/4/111/pdf?version=1743674936
- OA Status
- gold
- References
- 53
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4409169920
All OpenAlex metadata
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- OpenAlex ID
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https://openalex.org/W4409169920Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/inorganics13040111Digital Object Identifier
- Title
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Electrochemical Quartz Microbalance for Studying Electrodeposited Pt Catalysts for Methanol Oxidation ReactionWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-04-03Full publication date if available
- Authors
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Bangfeng Zong, Xiao Jun Pan, Bo Wei, Lifang Zhang, Xiaoyan Feng, C. Hou, Hai Yan, Wenju Xie, Guicheng Liu, Ye FengList of authors in order
- Landing page
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https://doi.org/10.3390/inorganics13040111Publisher landing page
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https://www.mdpi.com/2304-6740/13/4/111/pdf?version=1743674936Direct link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.mdpi.com/2304-6740/13/4/111/pdf?version=1743674936Direct OA link when available
- Concepts
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Electrochemistry, Catalysis, Quartz crystal microbalance, Methanol, Chemical engineering, Materials science, Quartz, Redox, Chemistry, Inorganic chemistry, Electrode, Organic chemistry, Metallurgy, Adsorption, Physical chemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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53Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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