Electrum, the Gold–Silver Alloy, from the Bulk Scale to the Nanoscale: Synthesis, Properties, and Segregation Rules Article Swipe
Grégory Guisbiers
,
Rubén Mendoza‐Cruz
,
Lourdes Bazán-Díaz
,
J. Jesús Velázquez‐Salazar
,
Rafael Mendoza
,
José Antonio Robledo-Torres
,
José Luis Rodríguez‐López
,
J.M. Montejano‐Carrizales
,
Robert L. Whetten
,
Miguel José–Yacamán
·
YOU?
·
· 2015
· Open Access
·
· DOI: https://doi.org/10.1021/acsnano.5b05755
YOU?
·
· 2015
· Open Access
·
· DOI: https://doi.org/10.1021/acsnano.5b05755
The alloy Au-Ag system is an important noble bimetallic phase, both historically (as "Electrum") and now especially in nanotechnology, as it is applied in catalysis and nanomedicine. To comprehend the structural characteristics and the thermodynamic stability of this alloy, a knowledge of its phase diagram is required that considers explicitly its size and shape (morphology) dependence. However, as the experimental determination remains quite challenging at the nanoscale, theoretical guidance can provide significant advantages. Using a regular solution model within a nanothermodynamic approach to evaluate the size effect on all the parameters (melting temperature, melting enthalpy, and interaction parameters in both phases), the nanophase diagram is predicted. Besides an overall shift downward, there is a "tilting" effect on the solidus-liquidus curves for some particular shapes exposing the (100) and (110) facets (cube, rhombic dodecahedron, and cuboctahedron). The segregation calculation reveals the preferential presence of silver at the surface for all the polyhedral shapes considered, in excellent agreement with the latest transmission electron microscopy observations and energy dispersive spectroscopy analysis. By reviewing the nature of the surface segregated element of different bimetallic nanoalloys, two surface segregation rules, based on the melting temperatures and surface energies, are deduced. Finally, the optical properties of Au-Ag nanoparticles, calculated within the discrete dipole approximation, show the control that can be achieved in the tuning of the local surface plasmon resonance, depending of the alloy content, the chemical ordering, the morphology, the size of the nanoparticle, and the nature of the surrounding environment.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acsnano.5b05755
- OA Status
- green
- Cited By
- 192
- References
- 67
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2343226991
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W2343226991Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1021/acsnano.5b05755Digital Object Identifier
- Title
-
Electrum, the Gold–Silver Alloy, from the Bulk Scale to the Nanoscale: Synthesis, Properties, and Segregation RulesWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2015Year of publication
- Publication date
-
2015-11-25Full publication date if available
- Authors
-
Grégory Guisbiers, Rubén Mendoza‐Cruz, Lourdes Bazán-Díaz, J. Jesús Velázquez‐Salazar, Rafael Mendoza, José Antonio Robledo-Torres, José Luis Rodríguez‐López, J.M. Montejano‐Carrizales, Robert L. Whetten, Miguel José–YacamánList of authors in order
- Landing page
-
https://doi.org/10.1021/acsnano.5b05755Publisher landing page
- Open access
-
YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
-
https://doi.org/10.1021/acsnano.5b05755Direct OA link when available
- Concepts
-
Materials science, Liquidus, Phase diagram, Bimetallic strip, Alloy, Nanoscopic scale, Solidus, Discrete dipole approximation, Nanoparticle, Noble metal, Phase (matter), Surface energy, Chemical physics, Nanotechnology, Dipole, Metal, Metallurgy, Composite material, Chemistry, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
192Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 11, 2024: 14, 2023: 21, 2022: 19, 2021: 22Per-year citation counts (last 5 years)
- References (count)
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67Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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