Enhanced hydrogen evolution reaction on hybrids of cobalt phosphide and molybdenum phosphide Article Swipe

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Si-Ling Fang , Tsu‐Chin Chou , Satyanarayana Samireddi , Kuei‐Hsien Chen , Li‐Chyong Chen , Wei‐Fu Chen ·

YOU? · · 2017 · Open Access · · DOI: https://doi.org/10.1098/rsos.161016

Production of hydrogen from water electrolysis has stimulated the search of sustainable electrocatalysts as possible alternatives. Recently, cobalt phosphide (CoP) and molybdenum phosphide (MoP) received great attention owing to their superior catalytic activity and stability towards the hydrogen evolution reaction (HER) which rivals platinum catalysts. In this study, we synthesize and study a series of catalysts based on hybrids of CoP and MoP with different Co/Mo ratio. The HER activity shows a volcano shape and reaches a maximum for Co/Mo = 1. Tafel analysis indicates a change in the dominating step of Volmer–Hyrovský mechanism. Interestingly, X-ray diffraction patterns confirmed a major ternary interstitial hexagonal CoMoP 2 crystal phase is formed which enhances the electrochemical activity.

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Phosphide Tafel equation Catalysis Hydrogen production Molybdenum Cobalt Materials science Ternary operation Hydrogen Platinum Electrochemistry Inorganic chemistry Chemical engineering Chemistry Metallurgy Physical chemistry Electrode Computer science Organic chemistry Engineering Programming language Biochemistry

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Type: article
Language: en
Landing Page: https://doi.org/10.1098/rsos.161016
OA Status: gold
Cited By: 20
References: 40
Related Works: 10
OpenAlex ID: https://openalex.org/W2593460661

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DOI: https://doi.org/10.1098/rsos.161016

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Title: Enhanced hydrogen evolution reaction on hybrids of cobalt phosphide and molybdenum phosphide

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Language: en

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Publication year: 2017

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Publication date: 2017-03-01

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Authors: Si-Ling Fang, Tsu‐Chin Chou, Satyanarayana Samireddi, Kuei‐Hsien Chen, Li‐Chyong Chen, Wei‐Fu Chen

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Landing page: https://doi.org/10.1098/rsos.161016

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Concepts: Phosphide, Tafel equation, Catalysis, Hydrogen production, Molybdenum, Cobalt, Materials science, Ternary operation, Hydrogen, Platinum, Electrochemistry, Inorganic chemistry, Chemical engineering, Chemistry, Metallurgy, Physical chemistry, Electrode, Computer science, Organic chemistry, Engineering, Programming language, Biochemistry

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Cited by: 20

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Citations by year (recent): 2025: 2, 2024: 1, 2023: 2, 2022: 1, 2021: 2

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