Enhanced Photoredox Activity of BiVO4/Prussian Blue Nanocomposites for Efficient Pollutant Removal from Aqueous Media under Low-Cost LEDs Illumination Article Swipe
Abrar Khan
,
Leonardo Marchiori
,
Elias Paiva Ferreira‐Neto
,
Heberton Wender
,
Rashida Parveen
,
Mohammad Muneeb
,
Bianca Oliveira Mattos
,
Ubirajara Pereira Rodrigues Filho
,
Sidney J. L. Ribeiro
,
Sajjad Ullah
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/catal12121612
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/catal12121612
Bismuth vanadate (BiVO4, BV) is a widely explored photocatalyst for photo(electro)chemical applications, but its full photocatalytic potential is hindered by the fast recombination and low mobility of photogenerated charge carriers. Herein, we propose the photodeposition of different amounts of Prussian blue (PB) cocatalysts on the surface of monoclinic BV to obtain BV-PB composite photocatalysts with increased photoactivity. The as-prepared BV and BV-PB composites were characterized by an array of analytic techniques such scanning eletron microscopy (SEM), transmission eletron microscopy (TEM), X-day diffraction (XRD), and spectroscopic techniques including Fourier-transform infrared spectroscopy (FTIR), diffuse reflectance spectroscopy (DRS), electrochemical impedance spectroscopy (EIS), photoluminescence (PL), and Raman spectroscopy. The addition of PB not only increases the absorption of visible light, as indicated by DRS, but also improves the charge carriers’ transfer across the photocatalysts/solution interface and hence reduces electron-hole (e−-h+) recombination, as confirmed by EIS and PL measurements. Resultantly, the BV-PB composite photocatalysts with optimum PB loading exhibited enhanced Cr(VI) photoreduction efficiency as compared to pristine BV under visible light illumination from low-power blue light-emitting diodes (LEDs), thanks to the cocatalyst role of PB which mediates the transfer of photoexcited conduction band (CB) electrons from BV to Cr(VI) species in solution. Moreover, as compared to pristine BV and BV + H2O2, a drastic increase in the methylene blue (MB) photo-oxidation efficiency was observed for BV-PB in the presence of a minute quantity of H2O2 due to a synergic effect between the photocatalytic and Fenton-like processes. While pure BV photodegraded around 70% of MB dye within 120 min, the BV-PB/H2O2 and BV/H2O2 system could degrade almost 100% of the dye within 20 min (kobs. = 0.375 min−1) and 40 min (kobs. = 0.055 min−1), respectively. The practical approach employed in this work may pioneer new prospects for synthesizing new BV-based photocatalytic systems with low production costs and high photoredox efficiencies.
Related Topics
Concepts
Bismuth vanadate
Photocatalysis
Dielectric spectroscopy
Diffuse reflectance infrared fourier transform
Prussian blue
Materials science
Fourier transform infrared spectroscopy
Visible spectrum
Photoluminescence
Photochemistry
Photocurrent
Spectroscopy
Chemistry
Charge carrier
Nuclear chemistry
Analytical Chemistry (journal)
Chemical engineering
Optoelectronics
Electrochemistry
Organic chemistry
Engineering
Quantum mechanics
Physics
Catalysis
Electrode
Physical chemistry
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/catal12121612
- https://www.mdpi.com/2073-4344/12/12/1612/pdf?version=1670837292
- OA Status
- gold
- Cited By
- 2
- References
- 65
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4311961533
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4311961533Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.3390/catal12121612Digital Object Identifier
- Title
-
Enhanced Photoredox Activity of BiVO4/Prussian Blue Nanocomposites for Efficient Pollutant Removal from Aqueous Media under Low-Cost LEDs IlluminationWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
-
2022-12-08Full publication date if available
- Authors
-
Abrar Khan, Leonardo Marchiori, Elias Paiva Ferreira‐Neto, Heberton Wender, Rashida Parveen, Mohammad Muneeb, Bianca Oliveira Mattos, Ubirajara Pereira Rodrigues Filho, Sidney J. L. Ribeiro, Sajjad UllahList of authors in order
- Landing page
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https://doi.org/10.3390/catal12121612Publisher landing page
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https://www.mdpi.com/2073-4344/12/12/1612/pdf?version=1670837292Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
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https://www.mdpi.com/2073-4344/12/12/1612/pdf?version=1670837292Direct OA link when available
- Concepts
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Bismuth vanadate, Photocatalysis, Dielectric spectroscopy, Diffuse reflectance infrared fourier transform, Prussian blue, Materials science, Fourier transform infrared spectroscopy, Visible spectrum, Photoluminescence, Photochemistry, Photocurrent, Spectroscopy, Chemistry, Charge carrier, Nuclear chemistry, Analytical Chemistry (journal), Chemical engineering, Optoelectronics, Electrochemistry, Organic chemistry, Engineering, Quantum mechanics, Physics, Catalysis, Electrode, Physical chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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2Total citation count in OpenAlex
- Citations by year (recent)
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2025: 1, 2023: 1Per-year citation counts (last 5 years)
- References (count)
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65Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.reduces | 133 |
| abstract_inverted_index.species | 194 |
| abstract_inverted_index.surface | 45 |
| abstract_inverted_index.systems | 296 |
| abstract_inverted_index.visible | 114, 164 |
| abstract_inverted_index.BV-based | 294 |
| abstract_inverted_index.Prussian | 39 |
| abstract_inverted_index.addition | 105 |
| abstract_inverted_index.analytic | 69 |
| abstract_inverted_index.approach | 282 |
| abstract_inverted_index.compared | 159, 199 |
| abstract_inverted_index.employed | 283 |
| abstract_inverted_index.enhanced | 154 |
| abstract_inverted_index.explored | 7 |
| abstract_inverted_index.hindered | 18 |
| abstract_inverted_index.improves | 122 |
| abstract_inverted_index.increase | 209 |
| abstract_inverted_index.infrared | 88 |
| abstract_inverted_index.mediates | 181 |
| abstract_inverted_index.min−1) | 271 |
| abstract_inverted_index.mobility | 25 |
| abstract_inverted_index.observed | 218 |
| abstract_inverted_index.presence | 223 |
| abstract_inverted_index.pristine | 161, 201 |
| abstract_inverted_index.quantity | 227 |
| abstract_inverted_index.scanning | 72 |
| abstract_inverted_index.synergic | 233 |
| abstract_inverted_index.transfer | 126, 183 |
| abstract_inverted_index.vanadate | 1 |
| abstract_inverted_index.(e−-h+) | 135 |
| abstract_inverted_index.Moreover, | 197 |
| abstract_inverted_index.carriers. | 29 |
| abstract_inverted_index.composite | 52, 147 |
| abstract_inverted_index.confirmed | 138 |
| abstract_inverted_index.different | 36 |
| abstract_inverted_index.electrons | 189 |
| abstract_inverted_index.exhibited | 153 |
| abstract_inverted_index.impedance | 96 |
| abstract_inverted_index.including | 86 |
| abstract_inverted_index.increased | 55 |
| abstract_inverted_index.increases | 110 |
| abstract_inverted_index.indicated | 117 |
| abstract_inverted_index.interface | 130 |
| abstract_inverted_index.low-power | 168 |
| abstract_inverted_index.methylene | 212 |
| abstract_inverted_index.min−1), | 278 |
| abstract_inverted_index.potential | 16 |
| abstract_inverted_index.practical | 281 |
| abstract_inverted_index.prospects | 290 |
| abstract_inverted_index.solution. | 196 |
| abstract_inverted_index.BV-PB/H2O2 | 254 |
| abstract_inverted_index.absorption | 112 |
| abstract_inverted_index.cocatalyst | 176 |
| abstract_inverted_index.composites | 62 |
| abstract_inverted_index.conduction | 186 |
| abstract_inverted_index.efficiency | 157, 216 |
| abstract_inverted_index.microscopy | 74, 78 |
| abstract_inverted_index.monoclinic | 47 |
| abstract_inverted_index.photoredox | 303 |
| abstract_inverted_index.processes. | 240 |
| abstract_inverted_index.production | 299 |
| abstract_inverted_index.techniques | 70, 85 |
| abstract_inverted_index.Fenton-like | 239 |
| abstract_inverted_index.as-prepared | 58 |
| abstract_inverted_index.carriers’ | 125 |
| abstract_inverted_index.cocatalysts | 42 |
| abstract_inverted_index.diffraction | 81 |
| abstract_inverted_index.reflectance | 92 |
| abstract_inverted_index.Resultantly, | 144 |
| abstract_inverted_index.illumination | 166 |
| abstract_inverted_index.photoexcited | 185 |
| abstract_inverted_index.spectroscopy | 89, 93, 97 |
| abstract_inverted_index.synthesizing | 292 |
| abstract_inverted_index.transmission | 76 |
| abstract_inverted_index.applications, | 11 |
| abstract_inverted_index.characterized | 64 |
| abstract_inverted_index.efficiencies. | 304 |
| abstract_inverted_index.electron-hole | 134 |
| abstract_inverted_index.measurements. | 143 |
| abstract_inverted_index.photocatalyst | 8 |
| abstract_inverted_index.photodegraded | 244 |
| abstract_inverted_index.recombination | 22 |
| abstract_inverted_index.respectively. | 279 |
| abstract_inverted_index.spectroscopic | 84 |
| abstract_inverted_index.spectroscopy. | 103 |
| abstract_inverted_index.light-emitting | 170 |
| abstract_inverted_index.photoactivity. | 56 |
| abstract_inverted_index.photocatalysts | 53, 148 |
| abstract_inverted_index.photocatalytic | 15, 237, 295 |
| abstract_inverted_index.photogenerated | 27 |
| abstract_inverted_index.photoreduction | 156 |
| abstract_inverted_index.recombination, | 136 |
| abstract_inverted_index.electrochemical | 95 |
| abstract_inverted_index.photo-oxidation | 215 |
| abstract_inverted_index.photodeposition | 34 |
| abstract_inverted_index.Fourier-transform | 87 |
| abstract_inverted_index.photoluminescence | 99 |
| abstract_inverted_index.photo(electro)chemical | 10 |
| abstract_inverted_index.photocatalysts/solution | 129 |
| cited_by_percentile_year.max | 95 |
| cited_by_percentile_year.min | 89 |
| corresponding_author_ids | https://openalex.org/A5081177468 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 10 |
| corresponding_institution_ids | https://openalex.org/I36001604 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/6 |
| sustainable_development_goals[0].score | 0.6800000071525574 |
| sustainable_development_goals[0].display_name | Clean water and sanitation |
| citation_normalized_percentile.value | 0.35745495 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |