Enhancement of dye-sensitized solar cell efficiency through co-sensitization of thiophene-based organic compounds and metal-based N-719 Article Swipe
Ismail Althagafi
,
Nashwa M. El‐Metwaly
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1016/j.arabjc.2021.103080
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1016/j.arabjc.2021.103080
Synthesis of five novel thiophene-based metal-free organic dyes, named IS1-5, to study their photophysical, electrochemical properties and photovoltaic performance as sensitizers and co-sensitizers for DSSCs. Dyes IS-5 are cyanoacetanilide derivatives, which are distinguished by their small size, the simple preparation method, and the presence of multiple anchoring species (CO and CN) within their molecular structure. From their UV/Vis. spectra, IS-4 and IS-5 displayed the highest molar extinction coefficient with a bathochromic-shift to the intramolecular charge transfer band. In addition, to recognize the potential of HOMO level and the potential of LUMO level among all IS1-5 dyes, the cyclic voltammetry technique must be used. Their characteristics assert that all dyes possess the qualifications essential to be used as a sensitizer for dye-sensitized solar cells (DSSCs). Interestingly, over co-sensitization, all dyes showed better photovoltage values (VOC) than the standard dye N-719. Among Dyes IS1-5, co-sensitizer IS-5 showed the highest photoconversion efficiency (η) of (8.09%) compared to the standard dye N-719 (7.61%). Moreover, electrochemical impedance spectroscopy (EIS) asserts the impact of this dye on improving charge transfer in TiO2. Finally, density functional theory (DFT) has been studied for dyes IS1-5 using Guassian09 software and the outcomes comfortably agree with experimental results.
Related Topics
Concepts
Chemistry
Dye-sensitized solar cell
Thiophene
HOMO/LUMO
Dielectric spectroscopy
Bathochromic shift
Photochemistry
Molar absorptivity
Cyclic voltammetry
Intramolecular force
Density functional theory
Electrochemistry
Physical chemistry
Molecule
Computational chemistry
Organic chemistry
Electrode
Fluorescence
Physics
Electrolyte
Optics
Quantum mechanics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.arabjc.2021.103080
- OA Status
- gold
- Cited By
- 37
- References
- 44
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3132681744
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3132681744Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.arabjc.2021.103080Digital Object Identifier
- Title
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Enhancement of dye-sensitized solar cell efficiency through co-sensitization of thiophene-based organic compounds and metal-based N-719Work title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-02-21Full publication date if available
- Authors
-
Ismail Althagafi, Nashwa M. El‐MetwalyList of authors in order
- Landing page
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https://doi.org/10.1016/j.arabjc.2021.103080Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1016/j.arabjc.2021.103080Direct OA link when available
- Concepts
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Chemistry, Dye-sensitized solar cell, Thiophene, HOMO/LUMO, Dielectric spectroscopy, Bathochromic shift, Photochemistry, Molar absorptivity, Cyclic voltammetry, Intramolecular force, Density functional theory, Electrochemistry, Physical chemistry, Molecule, Computational chemistry, Organic chemistry, Electrode, Fluorescence, Physics, Electrolyte, Optics, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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37Total citation count in OpenAlex
- Citations by year (recent)
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2025: 7, 2024: 12, 2023: 6, 2022: 10, 2021: 2Per-year citation counts (last 5 years)
- References (count)
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44Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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