Enhancement of single upconversion nanoparticle imaging by topologically segregated core-shell structure with inward energy migration Article Swipe
Yanxin Zhang
,
Rongrong Wen
,
Jialing Hu
,
Daoming Guan
,
Xiaochen Qiu
,
Yunxiang Zhang
,
Daniel S. Kohane
,
Qian Liu
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-022-33660-8
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-022-33660-8
Manipulating topological arrangement is a powerful tool for tuning energy migration in natural photosynthetic proteins and artificial polymers. Here, we report an inorganic optical nanosystem composed of NaErF 4 and NaYbF 4 , in which topological arrangement enhanced upconversion luminescence. Three architectures are designed for considerations pertaining to energy migration and energy transfer within nanoparticles: outside-in, inside-out, and local energy transfer. The outside-in architecture produces the maximum upconversion luminescence, around 6-times brighter than that of the inside-out at the single-particle level. Monte Carlo simulation suggests a topology-dependent energy migration favoring the upconversion luminescence of outside-in structure. The optimized outside-in structure shows more than an order of magnitude enhancement of upconversion brightness compared to the conventional core-shell structure at the single-particle level and is used for long-term single-particle tracking in living cells. Our findings enable rational nanoprobe engineering for single-molecule imaging and also reveal counter-intuitive relationships between upconversion nanoparticle structure and optical properties.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41467-022-33660-8
- https://www.nature.com/articles/s41467-022-33660-8.pdf
- OA Status
- gold
- Cited By
- 69
- References
- 69
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4303453492
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Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4303453492Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41467-022-33660-8Digital Object Identifier
- Title
-
Enhancement of single upconversion nanoparticle imaging by topologically segregated core-shell structure with inward energy migrationWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-10-07Full publication date if available
- Authors
-
Yanxin Zhang, Rongrong Wen, Jialing Hu, Daoming Guan, Xiaochen Qiu, Yunxiang Zhang, Daniel S. Kohane, Qian LiuList of authors in order
- Landing page
-
https://doi.org/10.1038/s41467-022-33660-8Publisher landing page
- PDF URL
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https://www.nature.com/articles/s41467-022-33660-8.pdfDirect link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
-
https://www.nature.com/articles/s41467-022-33660-8.pdfDirect OA link when available
- Concepts
-
Photon upconversion, Materials science, Luminescence, Nanoprobe, Nanoparticle, Brightness, Particle (ecology), Nanotechnology, Optoelectronics, Core (optical fiber), Topology (electrical circuits), Optics, Physics, Geology, Composite material, Mathematics, Combinatorics, OceanographyTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
69Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 28, 2024: 23, 2023: 18Per-year citation counts (last 5 years)
- References (count)
-
69Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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