Enhancing energetic disorder in all-organic composite dielectrics for high-temperature capacitive energy storage Article Swipe
Tan Zeng
,
Meng Li
,
Qiao Li
,
Dongduan Liu
,
Qian Zhou
,
Jinliang He
,
Qi Li
,
Chao Yuan
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-025-60741-1
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-025-60741-1
The urgent demand for capacitive energy storage at elevated temperatures is limited by significant leakage currents in existing polymer dielectrics, which lead to excessive heat generation and increase the risk of thermal runaway. Here we demonstrate a strategy to mitigate conduction loss by modulating energetic disorder within the polymer matrix. Incorporation of high-polarity organic molecules into polyetherimide enhances dipole-dipole interactions, increasing energetic disorder and thereby decreasing charge carrier mobility. Experimental measurements and computational simulations reveal that disorder-induced energy fluctuations broaden the energy separation between transport states, effectively suppressing charge transport. The resulting composite delivers an energy density of 6.45 J cm −3 with a charge-discharge efficiency of 90% at 200 °C, and exhibits stable performance over 100,000 cycles under an applied field of 400 MV m −1 . The observed uniformity and quality of the all-organic composite films address the challenges of scalable manufacturing for dielectric films, offering a practical pathway for the development of high-temperature dielectric materials.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41467-025-60741-1
- https://www.nature.com/articles/s41467-025-60741-1.pdf
- OA Status
- gold
- Cited By
- 24
- References
- 50
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4411887038
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4411887038Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41467-025-60741-1Digital Object Identifier
- Title
-
Enhancing energetic disorder in all-organic composite dielectrics for high-temperature capacitive energy storageWork title
- Type
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articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2025Year of publication
- Publication date
-
2025-07-01Full publication date if available
- Authors
-
Tan Zeng, Meng Li, Qiao Li, Dongduan Liu, Qian Zhou, Jinliang He, Qi Li, Chao YuanList of authors in order
- Landing page
-
https://doi.org/10.1038/s41467-025-60741-1Publisher landing page
- PDF URL
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https://www.nature.com/articles/s41467-025-60741-1.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
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https://www.nature.com/articles/s41467-025-60741-1.pdfDirect OA link when available
- Concepts
-
Materials science, Dielectric, Dipole, Capacitive sensing, Thermal conduction, Energy storage, Composite number, Optoelectronics, Chemical physics, Composite material, Electrical engineering, Chemistry, Thermodynamics, Organic chemistry, Power (physics), Engineering, PhysicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
24Total citation count in OpenAlex
- Citations by year (recent)
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2025: 24Per-year citation counts (last 5 years)
- References (count)
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50Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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