Estimating the Diffusion Coefficient of Lithium in Graphite: Extremely Fast Charging and a Comparison of Data Analysis Techniques Article Swipe
Minkyu Kim
,
David Robertson
,
Dennis W. Dees
,
Koffi P. C. Yao
,
Wenquan Lu
,
Stephen E. Trask
,
Joel T. Kirner
,
Ira Bloom
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1149/1945-7111/ac0d4f
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.1149/1945-7111/ac0d4f
Galvanostatic intermittent titration experiments were performed in three-electrode cells to characterize the effect of C/2, 2-C and 4-C charge rates on the observed lithium diffusion coefficient. As part of the data analysis process, we compared the classic Weppner-Huggins analysis of polarization data with a newer (Wang et al.) analysis method for depolarization data. At low values of x in Li x C 6 , both analysis methods showed the same general trend in the apparent lithium diffusion coefficient, 4-C > 2-C > C/2. The two techniques differed in the magnitude of the estimated diffusion coefficient by about a factor of 100. The observed increase in diffusion coefficient does not last over a large compositional range. Since the estimates from the method of Weppner and Huggins may contain artifacts due to the use of particulate electrodes and high charge rates, the method of Wang et al. may produce better values.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1149/1945-7111/ac0d4f
- OA Status
- green
- Cited By
- 25
- References
- 44
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3173964992
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W3173964992Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1149/1945-7111/ac0d4fDigital Object Identifier
- Title
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Estimating the Diffusion Coefficient of Lithium in Graphite: Extremely Fast Charging and a Comparison of Data Analysis TechniquesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-06-22Full publication date if available
- Authors
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Minkyu Kim, David Robertson, Dennis W. Dees, Koffi P. C. Yao, Wenquan Lu, Stephen E. Trask, Joel T. Kirner, Ira BloomList of authors in order
- Landing page
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https://doi.org/10.1149/1945-7111/ac0d4fPublisher landing page
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/1820106Direct OA link when available
- Concepts
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Diffusion, Lithium (medication), Analytical Chemistry (journal), Graphite, Electrode, Range (aeronautics), Titration, Polarization (electrochemistry), Chemistry, Materials science, Thermodynamics, Physics, Physical chemistry, Chromatography, Composite material, Medicine, Organic chemistry, EndocrinologyTop concepts (fields/topics) attached by OpenAlex
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25Total citation count in OpenAlex
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2025: 6, 2024: 5, 2023: 8, 2022: 3, 2021: 2Per-year citation counts (last 5 years)
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44Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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