Ether-compatible sulfurized polyacrylonitrile cathode with excellent performance enabled by fast kinetics via selenium doping Article Swipe
Xin Chen
,
Linfeng Peng
,
Lihui Wang
,
Jiaqiang Yang
,
Zhangxiang Hao
,
Jingwei Xiang
,
Kai Yuan
,
Yunhui Huang
,
Bin Shan
,
Lixia Yuan
,
Jia Xie
·
YOU?
·
· 2019
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-019-08818-6
YOU?
·
· 2019
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-019-08818-6
Sulfurized polyacrylonitrile is suggested to contain S n ( n ≤ 4) and shows good electrochemical performance in carbonate electrolytes for lithium sulfur batteries. However inferior results in ether electrolytes suggest that high solubility of Li 2 S n ( n ≤ 4) trumps the limited redox conversion, leading to dissolution and shuttling. Here, we introduce a small amount of selenium in sulfurized polyacrylonitrile to accelerate the redox conversion, delivering excellent performance in both carbonate and ether electrolytes, including high reversible capacity (1300 mA h g −1 at 0.2 A g −1 ), 84% active material utilization and high rate (capacity up to 900 mA h g −1 at 10 A g −1 ). These cathodes can undergo 800 cycles with nearly 100% Coulombic efficiency and ultralow 0.029% capacity decay per cycle. Polysulfide dissolution is successfully suppressed by enhanced reaction kinetics. This work demonstrates an ether compatible sulfur cathode involving intermediate Li 2 S n ( n ≤ 4), attractive rate and cycling performance, and a promising solution towards applicable lithium-sulfur batteries.
Related Topics
Concepts
Polysulfide
Polyacrylonitrile
Faraday efficiency
Dissolution
Electrolyte
Materials science
Electrochemistry
Cathode
Chemical engineering
Ether
Redox
Lithium (medication)
Inorganic chemistry
Sulfur
Selenium
Chemistry
Electrode
Organic chemistry
Polymer
Physical chemistry
Engineering
Endocrinology
Composite material
Metallurgy
Medicine
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41467-019-08818-6
- https://www.nature.com/articles/s41467-019-08818-6.pdf
- OA Status
- gold
- Cited By
- 309
- References
- 62
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2920715038
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W2920715038Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1038/s41467-019-08818-6Digital Object Identifier
- Title
-
Ether-compatible sulfurized polyacrylonitrile cathode with excellent performance enabled by fast kinetics via selenium dopingWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2019Year of publication
- Publication date
-
2019-03-04Full publication date if available
- Authors
-
Xin Chen, Linfeng Peng, Lihui Wang, Jiaqiang Yang, Zhangxiang Hao, Jingwei Xiang, Kai Yuan, Yunhui Huang, Bin Shan, Lixia Yuan, Jia XieList of authors in order
- Landing page
-
https://doi.org/10.1038/s41467-019-08818-6Publisher landing page
- PDF URL
-
https://www.nature.com/articles/s41467-019-08818-6.pdfDirect link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
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https://www.nature.com/articles/s41467-019-08818-6.pdfDirect OA link when available
- Concepts
-
Polysulfide, Polyacrylonitrile, Faraday efficiency, Dissolution, Electrolyte, Materials science, Electrochemistry, Cathode, Chemical engineering, Ether, Redox, Lithium (medication), Inorganic chemistry, Sulfur, Selenium, Chemistry, Electrode, Organic chemistry, Polymer, Physical chemistry, Engineering, Endocrinology, Composite material, Metallurgy, MedicineTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
309Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 45, 2024: 49, 2023: 58, 2022: 54, 2021: 51Per-year citation counts (last 5 years)
- References (count)
-
62Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.suggested | 4 |
| abstract_inverted_index.Sulfurized | 1 |
| abstract_inverted_index.accelerate | 66 |
| abstract_inverted_index.applicable | 170 |
| abstract_inverted_index.attractive | 160 |
| abstract_inverted_index.batteries. | 24, 172 |
| abstract_inverted_index.compatible | 147 |
| abstract_inverted_index.delivering | 70 |
| abstract_inverted_index.efficiency | 125 |
| abstract_inverted_index.reversible | 81 |
| abstract_inverted_index.shuttling. | 53 |
| abstract_inverted_index.solubility | 34 |
| abstract_inverted_index.sulfurized | 63 |
| abstract_inverted_index.suppressed | 137 |
| abstract_inverted_index.Polysulfide | 133 |
| abstract_inverted_index.conversion, | 48, 69 |
| abstract_inverted_index.dissolution | 51, 134 |
| abstract_inverted_index.performance | 17, 72 |
| abstract_inverted_index.utilization | 97 |
| abstract_inverted_index.demonstrates | 144 |
| abstract_inverted_index.electrolytes | 20, 30 |
| abstract_inverted_index.intermediate | 151 |
| abstract_inverted_index.performance, | 164 |
| abstract_inverted_index.successfully | 136 |
| abstract_inverted_index.electrolytes, | 78 |
| abstract_inverted_index.lithium-sulfur | 171 |
| abstract_inverted_index.electrochemical | 16 |
| abstract_inverted_index.polyacrylonitrile | 2, 64 |
| cited_by_percentile_year.max | 100 |
| cited_by_percentile_year.min | 99 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 11 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/6 |
| sustainable_development_goals[0].score | 0.4099999964237213 |
| sustainable_development_goals[0].display_name | Clean water and sanitation |
| citation_normalized_percentile.value | 0.9961033 |
| citation_normalized_percentile.is_in_top_1_percent | True |
| citation_normalized_percentile.is_in_top_10_percent | True |