Evaluating the diffusion of Kr in UO ₂ and ADOPT ^TM using time-of-flight elastic recoil detection analysis (ToF-erda) Article Swipe

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R.J.W. Frost , Denise Adorno Lopes , Kyle Johnson , Sobhan Patnaik , Johan Oscarsson , Maurício A. Sortica , Per Petersson , Daniel Primetzhofer ·

YOU? · · 2024 · Open Access · · DOI: https://doi.org/10.1080/00223131.2024.2423639

A combination of 300 keV Kr-84 ion implantation and Time-of-Flight Elastic Recoil Detection Analysis is utilised to investigate the diffusion of Kr in UO2 and ADOPT (TM) fuels. Composition depth-profiles on the nanometer scale were obtained, both for as-implanted samples and after annealing at 800 degrees C for 1 h. Observed drifts in the 84Kr profiles could be associated with short-range diffusion mechanisms. The approach employed here provides the possibility to make direct comparisons with atomistic scale modelling data, and can be of service as a separate effect test in line with the Accelerated Fuel Qualification initiative.

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Elastic recoil detection Recoil Nuclear physics Diffusion Time of flight Physics Radiochemistry Atomic physics Materials science Chemistry Nanotechnology Thermodynamics Thin film Optics

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Type: article
Language: en
Landing Page: https://doi.org/10.1080/00223131.2024.2423639
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Cited By: 1
References: 27
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OpenAlex ID: https://openalex.org/W4404464273

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DOI: https://doi.org/10.1080/00223131.2024.2423639

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Title: Evaluating the diffusion of Kr in UO ₂ and ADOPT ^TM using time-of-flight elastic recoil detection analysis (ToF-erda)

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Language: en

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Publication year: 2024

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Publication date: 2024-11-18

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Authors: R.J.W. Frost, Denise Adorno Lopes, Kyle Johnson, Sobhan Patnaik, Johan Oscarsson, Maurício A. Sortica, Per Petersson, Daniel Primetzhofer

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Landing page: https://doi.org/10.1080/00223131.2024.2423639

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Concepts: Elastic recoil detection, Recoil, Nuclear physics, Diffusion, Time of flight, Physics, Radiochemistry, Atomic physics, Materials science, Chemistry, Nanotechnology, Thermodynamics, Thin film, Optics

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Cited by: 1

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Evaluating the diffusion of Kr in UO 2 and ADOPT TM using time-of-flight elastic recoil detection analysis (ToF-erda) Article Swipe

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Evaluating the diffusion of Kr in UO ₂ and ADOPT ^TM using time-of-flight elastic recoil detection analysis (ToF-erda) Article Swipe