Everything is imperfect: Studies on point defects in insulators Article Swipe
Point defects can be detrimental or absolutely necessary for the performance of a material. Due to the implications defectshave on a material, defects have been widely studied over the last century. However, there are plenty of open questions that concernsthe effect of point defects in materials but also properties of defects that are common across materials. This thesis consists of studies on equilibrium properties of oxygen vacancies and optical lineshapes of transitions on point defects. Using first principles calculations, general properties of oxygen vacancies in wide band gap oxides are revealed. The induced defect level of the oxygen vacancy is found to be constant in a number of materials. It is often located in the middle of the band gap and associated with a large structural distortion upon a change in charge state. Due to the large structural distortion, oxygen vacancies may play a role in luminescence quenching in oxide based phosphors and recombination processes in general. A possible recombination mechanism involving oxygen vacancies is proposed in the oxide phosphor Ce:YAG, which could explain the luminescence quenching. In connection with luminescence quenching in Ce:YAG, the origin of the phonon side bands of the optical transition is elucidated. Due to the connection between the optical lineshape and the geometry of a point defect, the optical lineshape can be used to identify point defects. The point defect emission in hexagonal boron nitride is addressed and several point defects can be matched to observed emission lines.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://research.chalmers.se/en/publication/516667
- https://research.chalmers.se/en/publication/516667
- OA Status
- green
- Related Works
- 19
- OpenAlex ID
- https://openalex.org/W3020604484
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3020604484Canonical identifier for this work in OpenAlex
- Title
-
Everything is imperfect: Studies on point defects in insulatorsWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
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2020Year of publication
- Publication date
-
2020-01-01Full publication date if available
- Authors
-
Christopher LinderälvList of authors in order
- Landing page
-
https://research.chalmers.se/en/publication/516667Publisher landing page
- PDF URL
-
https://research.chalmers.se/en/publication/516667Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
- OA URL
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https://research.chalmers.se/en/publication/516667Direct OA link when available
- Concepts
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Crystallographic defect, Luminescence, Materials science, Quenching (fluorescence), Band gap, Vacancy defect, Oxide, Phosphor, Photoluminescence, Oxygen, Condensed matter physics, Optoelectronics, Molecular physics, Optics, Chemistry, Physics, Fluorescence, Metallurgy, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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19Other works algorithmically related by OpenAlex
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| abstract_inverted_index.associated | 121 |
| abstract_inverted_index.connection | 178, 200 |
| abstract_inverted_index.distortion | 126 |
| abstract_inverted_index.lineshapes | 69 |
| abstract_inverted_index.materials. | 55, 108 |
| abstract_inverted_index.principles | 77 |
| abstract_inverted_index.properties | 48, 63, 80 |
| abstract_inverted_index.quenching. | 176 |
| abstract_inverted_index.structural | 125, 137 |
| abstract_inverted_index.transition | 194 |
| abstract_inverted_index.concernsthe | 39 |
| abstract_inverted_index.defectshave | 18 |
| abstract_inverted_index.detrimental | 4 |
| abstract_inverted_index.distortion, | 138 |
| abstract_inverted_index.elucidated. | 196 |
| abstract_inverted_index.equilibrium | 62 |
| abstract_inverted_index.performance | 10 |
| abstract_inverted_index.transitions | 71 |
| abstract_inverted_index.implications | 17 |
| abstract_inverted_index.luminescence | 146, 175, 180 |
| abstract_inverted_index.calculations, | 78 |
| abstract_inverted_index.recombination | 153, 159 |
| cited_by_percentile_year | |
| corresponding_author_ids | https://openalex.org/A5039981124 |
| countries_distinct_count | 0 |
| institutions_distinct_count | 1 |
| citation_normalized_percentile.value | 0.05814391 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |