Experimental High-Resolution Observation of the Truncated Double-Icosahedron Structure: A Stable Twinned Shell in Alloyed Au–Ag Core@Shell Nanoparticles Article Swipe
Rubén Mendoza‐Cruz
,
Juan Pedro Palomares-Báez
,
S. López-López
,
J.M. Montejano‐Carrizales
,
José Luis Rodríguez‐López
,
Miguel José–Yacamán
,
Lourdes Bazán-Díaz
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1021/acs.nanolett.3c04435
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1021/acs.nanolett.3c04435
Given the binary nature of nanoalloy systems, their properties are dependent on their size, shape, structure, composition, and chemical ordering. When energy and entropic factors for shapes and structure variations are considered in nanoparticle growth, the spectra of shapes become so vast that even metastable arrangements have been reported under ambient conditions. Experimental and theoretical variations of multiply twinned particles have been observed, from the Ino and Marks decahedra to polyicosahedra and polydecahedra with comparable energetic stability among them. Herein, we report the experimental production of a stable doubly truncated double-icosahedron structure (TdIh) in Au-Ag nanoparticles, in which a twinned Ag-rich alloyed shell is reconstructed on a Au-Ag alloyed Ino-decahedral core. The structure, chemical composition, and growth pathway are proposed on the basis of high-angle annular dark-field scanning transmission electron microscopy analysis and excess energy calculations, while its structural stability is estimated by large-scale atomic molecular dynamics simulations. This novel nanostructure differs from other structures previously reported.
Related Topics
Concepts
Metastability
Nanostructure
Materials science
Nanoparticle
Shell (structure)
Transmission electron microscopy
Chemical physics
Scanning transmission electron microscopy
High-resolution transmission electron microscopy
Molecular dynamics
Atomic units
Crystallography
Molecular physics
Nanotechnology
Chemistry
Computational chemistry
Physics
Composite material
Organic chemistry
Quantum mechanics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acs.nanolett.3c04435
- https://pubs.acs.org/doi/pdf/10.1021/acs.nanolett.3c04435
- OA Status
- hybrid
- Cited By
- 5
- References
- 83
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4393380829
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4393380829Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acs.nanolett.3c04435Digital Object Identifier
- Title
-
Experimental High-Resolution Observation of the Truncated Double-Icosahedron Structure: A Stable Twinned Shell in Alloyed Au–Ag Core@Shell NanoparticlesWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-04-01Full publication date if available
- Authors
-
Rubén Mendoza‐Cruz, Juan Pedro Palomares-Báez, S. López-López, J.M. Montejano‐Carrizales, José Luis Rodríguez‐López, Miguel José–Yacamán, Lourdes Bazán-DíazList of authors in order
- Landing page
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https://doi.org/10.1021/acs.nanolett.3c04435Publisher landing page
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https://pubs.acs.org/doi/pdf/10.1021/acs.nanolett.3c04435Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
hybridOpen access status per OpenAlex
- OA URL
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https://pubs.acs.org/doi/pdf/10.1021/acs.nanolett.3c04435Direct OA link when available
- Concepts
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Metastability, Nanostructure, Materials science, Nanoparticle, Shell (structure), Transmission electron microscopy, Chemical physics, Scanning transmission electron microscopy, High-resolution transmission electron microscopy, Molecular dynamics, Atomic units, Crystallography, Molecular physics, Nanotechnology, Chemistry, Computational chemistry, Physics, Composite material, Organic chemistry, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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5Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 2, 2024: 3Per-year citation counts (last 5 years)
- References (count)
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83Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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