Exploring the Effects of Nano-CaCO3 on the Core–Shell Structure and Properties of HDPE/POE/Nano-CaCO3 Ternary Nanocomposites Article Swipe
Wei Liu
,
Lumin Wang
,
Xun Zhang
,
Hongliang Huang
,
Yongli Liu
,
Minghua Min
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.3390/polym16081146
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.3390/polym16081146
To address the dilemma of the stiffness and toughness properties of high-density polyethylene (HDPE) composites, titanate coupling agent-treated CaCO3 nanoparticles (nano-CaCO3) and ethylene–octene copolymer (POE) were utilized to blend with HDPE to prepare ternary nanocomposites via a two-sequence-step process. Meanwhile, a one-step process was also studied as a control. The obtained ternary nanocomposites were characterized by scanning electron microscopy (SEM), Advanced Rheometrics Expansion System (ARES), Dynamic Mechanical Analysis (DMA), wide-angle X-ray diffraction analysis (WXRD), and mechanical test. The SEM results showed one or two CaCO3 nanoparticles were well-encapsulated by POE and were uniformly dispersed into the HDPE matrix to form a core–shell structure of 100–200 nm in size by the two-step process, while CaCO3 nanoparticles were aggregated in the HDPE matrix by the one-step method. The result of the XRD showed that the nano-CaCO3 particle played a role in promoting crystallization in HDPE nanocomposites. Mechanical tests showed that the synergistic effect of both the POE elastomer and CaCO3 nanoparticles should account for the balanced performance of the ternary composites. In comparison with neat HDPE, the notched impact toughness of the ternary nanocomposites of HDPE/POE/nano-CaCO3 was significantly increased. In addition, the core–shell structure absorbed the fracture impact energy and prevent further propagation of micro-cracks, thus obtaining a higher notched Izod impact strength.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/polym16081146
- https://www.mdpi.com/2073-4360/16/8/1146/pdf?version=1713510770
- OA Status
- gold
- Cited By
- 3
- References
- 40
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4394956854
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4394956854Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.3390/polym16081146Digital Object Identifier
- Title
-
Exploring the Effects of Nano-CaCO3 on the Core–Shell Structure and Properties of HDPE/POE/Nano-CaCO3 Ternary NanocompositesWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-04-19Full publication date if available
- Authors
-
Wei Liu, Lumin Wang, Xun Zhang, Hongliang Huang, Yongli Liu, Minghua MinList of authors in order
- Landing page
-
https://doi.org/10.3390/polym16081146Publisher landing page
- PDF URL
-
https://www.mdpi.com/2073-4360/16/8/1146/pdf?version=1713510770Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
-
https://www.mdpi.com/2073-4360/16/8/1146/pdf?version=1713510770Direct OA link when available
- Concepts
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Nano-, Nanocomposite, Ternary operation, Materials science, High-density polyethylene, Shell (structure), Core (optical fiber), Nanoparticle, Nanotechnology, Composite material, Polyethylene, Computer science, Programming languageTop concepts (fields/topics) attached by OpenAlex
- Cited by
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3Total citation count in OpenAlex
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2025: 3Per-year citation counts (last 5 years)
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40Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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