Exploring the Photophysical Processes of an Al3+ Sensor Based on Schiff Base Article Swipe
Bingqing Sun
,
Haoyang Song
,
Yi Nan
,
Lei Liu
,
Juyoung Yoon
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/cphc.202500196
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/cphc.202500196
Schiff bases are commonly used as building blocks in the development of turn‐on sensors for Al 3+ detection. The isomerization of the CN bond in Schiff bases is generally believed to induce fluorescence quenching. Inhibiting this isomerization process through interactions with the target ion, Al 3+ , enhances fluorescence, enabling its detection. This mechanism is widely used to explain turn‐on signals in similar sensors. However, the photophysical processes of such sensors may be more complex, necessitating a deeper understanding of their underlying sensing mechanisms. This study presents a comprehensive investigation into the photophysical processes and sensing mechanism of a turn‐on sensor for Al 3+ featuring a Schiff base moiety. Multiple excited‐state intramolecular proton transfer (ESIPT) processes are observed, all closely associated with the Schiff base structure. These ESIPT processes trigger CN isomerization, leading to the formation of two nonemissive twisted intramolecular charge transfer (TICT) states. In addition to CN isomerization, two bond rotation processes with lower energy barriers are identified. These rotational processes generate two additional nonemissive TICT states and play a dominant role in the weak fluorescence of the sensor. This elucidation of photophysical processes provides a clearer understanding of the Al 3+ sensing mechanism.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/cphc.202500196
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cphc.202500196
- OA Status
- hybrid
- Cited By
- 1
- References
- 44
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4412021118
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Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4412021118Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/cphc.202500196Digital Object Identifier
- Title
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Exploring the Photophysical Processes of an Al3+ Sensor Based on Schiff BaseWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-07-04Full publication date if available
- Authors
-
Bingqing Sun, Haoyang Song, Yi Nan, Lei Liu, Juyoung YoonList of authors in order
- Landing page
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https://doi.org/10.1002/cphc.202500196Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cphc.202500196Direct link to full text PDF
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cphc.202500196Direct OA link when available
- Concepts
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Isomerization, Schiff base, Intramolecular force, Photochemistry, Chemistry, Moiety, Fluorescence, Quenching (fluorescence), Excited state, Stereochemistry, Catalysis, Organic chemistry, Nuclear physics, Physics, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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1Total citation count in OpenAlex
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2025: 1Per-year citation counts (last 5 years)
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44Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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