Exploring the Synergistic Interaction between Nickel- and Ruthenium-Based Catalysts for Carbon Dioxide Methanation Reaction Article Swipe
Juan Carlos Navarro de Miguel
,
Luis F. Bobadilla
,
M.Á. Centeno
,
O.H. Laguna
,
J.A. Odriozola
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1021/acssuschemeng.4c10845
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1021/acssuschemeng.4c10845
The utilization of nickel-ruthenium as bimetallic catalysts is widely recognized for its efficacy in enhancing the catalytic performance in the carbon dioxide methanation reaction. The present study focuses on the synergistic interplay between both active sites and their respective roles in the reaction mechanism through operando DRIFT-MS analysis. Findings reveal that the bimetallic catalyst is constituted by NiRu nanocrystallites with Ru atoms segregated at defect edge/corner sites, promoting the dissociation of carbon dioxide and the formation of CHx species. Furthermore, Ni atoms predominantly occupy facets or terrace sites, characterized by higher electron density conducive to carbon monoxide hydrogenation to methane. This research offers a comprehensive elucidation of the carbon dioxide methanation mechanism within a bimetallic system and underscores the efficacy of the operando methodology in advancing our fundamental understanding of heterogeneous catalysis.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acssuschemeng.4c10845
- OA Status
- green
- Cited By
- 2
- References
- 72
- Related Works
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- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4410943237Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acssuschemeng.4c10845Digital Object Identifier
- Title
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Exploring the Synergistic Interaction between Nickel- and Ruthenium-Based Catalysts for Carbon Dioxide Methanation ReactionWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-06-02Full publication date if available
- Authors
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Juan Carlos Navarro de Miguel, Luis F. Bobadilla, M.Á. Centeno, O.H. Laguna, J.A. OdriozolaList of authors in order
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https://doi.org/10.1021/acssuschemeng.4c10845Publisher landing page
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://hdl.handle.net/10261/398146Direct OA link when available
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Methanation, Ruthenium, Catalysis, Nickel, Carbon dioxide, Chemistry, Carbon fibers, Chemical engineering, Inorganic chemistry, Materials science, Organic chemistry, Composite number, Engineering, Composite materialTop concepts (fields/topics) attached by OpenAlex
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2Total citation count in OpenAlex
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2025: 2Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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