Extracting RABBITT-like phase information from time-dependent transient absorption spectra Article Swipe
Jan Jakob
,
C Bauer
,
M.-J. Ilhan
,
Divya Bharti
,
Christian Ott
,
Thomas Pfeifer
,
Klaus Bartschat
,
Anne Harth
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1103/physrevresearch.7.023244
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1103/physrevresearch.7.023244
We explore how the spectral phase of attosecond pulse trains influences the optical cross section in transient absorption (TA) spectroscopy. The interaction of extreme ultraviolet (XUV) and time-delayed near-infrared (NIR) fields with an atomic or molecular system governs the dynamics. As already shown in RABBITT experiments (Reconstruction of Attosecond Beating by Interference of Two-Photon Transitions), the spectral phase of the XUV pulses can be extracted from the photoionization spectrum as a function of the time delay. Similarly, this XUV phase imprints itself on delay-dependent optical cross-section oscillations. With a perturbative analytical approach and by simulating the quantum dynamics both in a few-level model and via solving the time-dependent Schrödinger equation for atomic hydrogen, we reveal the similarity between the spectral phase in RABBITT and TA spectroscopy.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1103/physrevresearch.7.023244
- http://link.aps.org/pdf/10.1103/PhysRevResearch.7.023244
- OA Status
- gold
- References
- 24
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4411208328
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Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4411208328Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1103/physrevresearch.7.023244Digital Object Identifier
- Title
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Extracting RABBITT-like phase information from time-dependent transient absorption spectraWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-06-11Full publication date if available
- Authors
-
Jan Jakob, C Bauer, M.-J. Ilhan, Divya Bharti, Christian Ott, Thomas Pfeifer, Klaus Bartschat, Anne HarthList of authors in order
- Landing page
-
https://doi.org/10.1103/physrevresearch.7.023244Publisher landing page
- PDF URL
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https://link.aps.org/pdf/10.1103/PhysRevResearch.7.023244Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
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https://link.aps.org/pdf/10.1103/PhysRevResearch.7.023244Direct OA link when available
- Concepts
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Transient (computer programming), Ultrafast laser spectroscopy, Phase (matter), Spectral line, Absorption spectroscopy, Materials science, Physics, Optics, Computer science, Quantum mechanics, Laser, Operating systemTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
- References (count)
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24Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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