Flexibility and Dynamicity Enhances and Controls Supramolecular Self‐Assembly of Zinc(II) Metallogels Article Swipe
Merlin R. Stühler
,
Hesam Makki
,
Dorothee Silbernagl
,
Mathias Dimde
,
Kai Ludwig
,
Bengt E. Tegner
,
Christopher Greve
,
Konstantin Rausch
,
Eva M. Herzig
,
Anna Köhler
,
Alex J. Plajer
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202507793
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adfm.202507793
Supramolecular self‐assembly of stacked architectures is typically achieved through hydrogen bonding or π–π interactions between monomers constructed from stable and inert bonds. In contrast, coordinative interactions of early metals promise distinct self‐assembly behaviour due to more flexible bonding geometries and a wider range of stabilities and exchange kinetics. In this report we demonstrate that tailoring the flexible coordination sphere of Zinc(II) complexes via subtle ligand modification promotes not only one but also three‐dimensional self‐assembly both thermodynamically and kinetically into higher‐order fibrous morphologies, the latter being elucidated by electron tomography. As a result, coordination chemistry can be translated into both nanoscopic (fibre stiffness) and macroscopic (thermal gel stability) material properties. Utilizing dynamicity enables gelation via subcomponent self‐assembly, constructing the supramolecular polymer network simultaneously with the monomer. Furthermore, coordinative dis‐ and reassembly via metal‐ligand exchange reactions involving the first and second coordination spheres allows for control over gelation and emission of the system. Our report links concepts in supramolecular self‐assembly and coordination chemistry by leveraging the unique bonding interactions that cannot be achieved for traditional monomers, promising applications in stimuli‐responsive optoelectronics.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adfm.202507793
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202507793
- OA Status
- hybrid
- References
- 62
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4410934666
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https://openalex.org/W4410934666Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adfm.202507793Digital Object Identifier
- Title
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Flexibility and Dynamicity Enhances and Controls Supramolecular Self‐Assembly of Zinc(II) MetallogelsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-06-01Full publication date if available
- Authors
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Merlin R. Stühler, Hesam Makki, Dorothee Silbernagl, Mathias Dimde, Kai Ludwig, Bengt E. Tegner, Christopher Greve, Konstantin Rausch, Eva M. Herzig, Anna Köhler, Alex J. PlajerList of authors in order
- Landing page
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https://doi.org/10.1002/adfm.202507793Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202507793Direct link to full text PDF
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202507793Direct OA link when available
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Supramolecular chemistry, Materials science, Zinc, Flexibility (engineering), Self-assembly, Nanotechnology, Supramolecular assembly, Crystallography, Crystal structure, Metallurgy, Chemistry, Statistics, MathematicsTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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