Four-Wave-Mixing Approach to In Situ Detection of Nanoparticles Article Swipe

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Alexandros Gerakis , Yao‐Wen Yeh , Mikhail N. Shneider , James Mitrani , B. Stratton , Yevgeny Raitses ·

YOU? · · 2018 · Open Access · · DOI: https://doi.org/10.1103/physrevapplied.9.014031

Here, we report on the development and experimental validation of a laser-based technique which uses coherent Rayleigh-Brillouin scattering (CRBS) to detect nanoparticles with characteristic sizes ranging from the atomic scale to tens of nanometers. This technique is aimed (nonexclusively) at the detection of nanoparticles produced by volumetric nanoparticle synthesis methods. Using CRBS, carbon nanoparticles of dimensions less than 10 nm and concentrations of 10¹⁰ cm^–3 are detected in situ in a carbon arc discharge with graphite electrodes. This four-wave-mixing approach should enable advances in the understanding of nanoparticle growth that could potentially lead to improved modeling of the growth mechanisms, and thus to improve synthesis selectivity of nanoparticles and yield.

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Imaging phantom Nanoparticle Rayleigh scattering Mixing (physics) Nucleation Physics Materials science Optics Atomic physics Nanotechnology Thermodynamics Quantum mechanics

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Type: article
Language: en
Landing Page: https://doi.org/10.1103/physrevapplied.9.014031
OA Status: green
Cited By: 24
References: 47
Related Works: 10
OpenAlex ID: https://openalex.org/W2787344504

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DOI: https://doi.org/10.1103/physrevapplied.9.014031

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Title: Four-Wave-Mixing Approach to In Situ Detection of Nanoparticles

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Type: article

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Language: en

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Publication year: 2018

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Publication date: 2018-01-29

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Authors: Alexandros Gerakis, Yao‐Wen Yeh, Mikhail N. Shneider, James Mitrani, B. Stratton, Yevgeny Raitses

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Landing page: https://doi.org/10.1103/physrevapplied.9.014031

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OA status: green

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OA URL: https://www.osti.gov/biblio/1418392

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Concepts: Imaging phantom, Nanoparticle, Rayleigh scattering, Mixing (physics), Nucleation, Physics, Materials science, Optics, Atomic physics, Nanotechnology, Thermodynamics, Quantum mechanics

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Cited by: 24

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