Frameworked electrolytes: Ionic transport behavior and high mobility for solid state batteries Article Swipe
Jianguo Sun
,
Hao Yuan
,
Jing Yang
,
Tuo Wang
,
Yulin Gao
,
Qi Zhao
,
Ximeng Liu
,
Haimei Wang
,
Yong‐Wei Zhang
,
John Wang
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/inf2.12487
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/inf2.12487
All solid‐state batteries (ASSBs) are the holy grails of rechargeable batteries, where extensive searches are ongoing in the pursuit of ideal solid‐state electrolytes. Nevertheless, there is still a long way off to the satisfactorily high (enough) ionic conductivity, long‐term stability and especially being able to form compatible interfaces with the solid electrodes. Herein, we have explored ionic transport behavior and high mobility in the sub‐nano pore networks in the framework structures. Macroscopically, the frameworked electrolyte behaves as a solid, and however in the (sub)‐nano scales, the very limited number of solvent molecules in confinement makes them completely different from that in liquid electrolyte. Differentiated from a liquid‐electrolyte counterpart, the interactions between the mobile ions and surrounding molecules are subject to dramatic changes, leading to a high ionic conductivity at room temperature with a low activation energy. Li + ions in the sub‐nano cages of the network structure are highly mobile and diffuse rather independently, where the rate‐limiting step of ions crossing cages is driven by the local concentration gradient and the electrostatic interactions between Li + ions. This new class of frameworked electrolytes (FEs) with both high ionic conductivity and desirable interface with solid electrodes are demonstrated to work with Li‐ion batteries, where the ASSB with LiFePO 4 shows a highly stable electrochemical performance of over 450 cycles at 2°C at room temperature, with an almost negligible capacity fade of 0.03‰ each cycle. In addition, the FE shows outstanding flexibility and anti‐flammability, which are among the key requirements of large‐scale applications. image
Related Topics
Concepts
Electrolyte
Ionic conductivity
Ion
Materials science
Chemical physics
Ionic bonding
Fast ion conductor
Ionic liquid
Electrochemistry
Conductivity
Electrode
Nanotechnology
Chemical engineering
Chemistry
Physical chemistry
Organic chemistry
Catalysis
Engineering
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/inf2.12487
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/inf2.12487
- OA Status
- gold
- Cited By
- 19
- References
- 52
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4389886189
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4389886189Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/inf2.12487Digital Object Identifier
- Title
-
Frameworked electrolytes: Ionic transport behavior and high mobility for solid state batteriesWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-12-18Full publication date if available
- Authors
-
Jianguo Sun, Hao Yuan, Jing Yang, Tuo Wang, Yulin Gao, Qi Zhao, Ximeng Liu, Haimei Wang, Yong‐Wei Zhang, John WangList of authors in order
- Landing page
-
https://doi.org/10.1002/inf2.12487Publisher landing page
- PDF URL
-
https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/inf2.12487Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/inf2.12487Direct OA link when available
- Concepts
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Electrolyte, Ionic conductivity, Ion, Materials science, Chemical physics, Ionic bonding, Fast ion conductor, Ionic liquid, Electrochemistry, Conductivity, Electrode, Nanotechnology, Chemical engineering, Chemistry, Physical chemistry, Organic chemistry, Catalysis, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
19Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 9, 2024: 10Per-year citation counts (last 5 years)
- References (count)
-
52Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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