Full-color tuning in multi-layer core-shell nanoparticles from single-wavelength excitation Article Swipe

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Jinshu Huang , Lili Tao , Haopeng Wei , Haozhang Huang , Jeong Woo Han , Bo Zhou ·

YOU? · · 2025 · Open Access · · DOI: https://doi.org/10.1038/s41467-025-57622-y

Lanthanide-based luminescent materials have shown great capabilities in addressing scientific problems encountered in diverse fields. However, achieving full-color switchable output under single-wavelength irradiation has remained a daunting challenge. Here we report a conceptual model to realize this aim by the temporal control of full upconversion evolution in a multi-layer core-shell nanostructure upon a single commercial 980-nm laser, instead of two or more excitation wavelengths as reported previously. We show that it is able to realize the red-to-green color change (from Er³⁺) under non-steady state excitation by constructing the cooperative modulation effect in the Er-Tm-Yb triple system, and single out the blue light (from Tm³⁺) by filtering out the short-decay emissions via a time-gating technique. The key role of Tm³⁺ in manipulating up-transition dynamics of Er³⁺ is further demonstrated. Our results present a deep insight into the photophysics of lanthanides, and help develop new generation of smart luminescent materials toward emerging photonic applications.

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Excitation Excitation wavelength Shell (structure) Core (optical fiber) Wavelength Materials science Layer (electronics) Nanoparticle Optoelectronics Nanotechnology Physics Composite material Quantum mechanics

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Type: article
Language: en
Landing Page: https://doi.org/10.1038/s41467-025-57622-y
PDF: https://www.nature.com/articles/s41467-025-57622-y.pdf
OA Status: gold
Cited By: 24
References: 48
Related Works: 10
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DOI: https://doi.org/10.1038/s41467-025-57622-y

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Title: Full-color tuning in multi-layer core-shell nanoparticles from single-wavelength excitation

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Language: en

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Publication year: 2025

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Publication date: 2025-03-11

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Authors: Jinshu Huang, Lili Tao, Haopeng Wei, Haozhang Huang, Jeong Woo Han, Bo Zhou

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Landing page: https://doi.org/10.1038/s41467-025-57622-y

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Concepts: Excitation, Excitation wavelength, Shell (structure), Core (optical fiber), Wavelength, Materials science, Layer (electronics), Nanoparticle, Optoelectronics, Nanotechnology, Physics, Composite material, Quantum mechanics

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Cited by: 24

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