Fully bio-based furan/maleic anhydride epoxy resin with enhanced adhesive properties Article Swipe
Noemi Faggio
,
A. Marotta
,
Veronica Ambrogi
,
Pierfrancesco Cerruti
,
Gennaro Gentile
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1007/s10853-023-08458-8
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1007/s10853-023-08458-8
Epoxy resins are widely used in a variety of application fields, thanks to their good mechanical strength, chemical resistance and adhesion to several substrates. Nowadays, the quite majority of epoxy resins are based on derivatives of bisphenol A (BPA), which poses serious health concerns. This issue is pushing the research towards suitable bio-based alternatives to this product, being furan-based epoxies very promising in this respect. In a previous work, 2,5-bis[(oxiran-2-ylmethoxy)methyl]furan (BOMF) was cured with methyl nadic anhydride (MNA), and successfully used as tinplate coating. Herein, in a view of increasing the sustainability of these epoxy resins, we have replaced MNA with maleic anhydride (MA), which can be derived from vegetable feedstocks, thus obtaining a fully bio-based epoxy resin. This latter has then been used as adhesive for carbon fiber-reinforced thermosetting plastics (CFRP). The curing process of the resin was monitored by differential scanning calorimetry (DSC) and chemo-rheological analysis. The results highlighted the significantly higher reactivity of BOMF towards MA compared to the diglycidyl ether of BPA (DGEBA). The crosslinked samples were characterized in their thermal, mechanical and adhesive properties. In comparison to DGEBA/MA and BOMF/MNA, BOMF/MA showed higher ultimate strain and slightly lower glass transition temperature, tensile modulus and ultimate strength. Interestingly, BOMF/MA displayed outstanding adhesive strength on CFRP joints, outperforming the DGEBA-based counterpart by three times. Indeed, by properly selecting the anhydride curing agent, a highly ductile fully bio-based material was developed for high performance adhesive applications. The overall results demonstrate that the properties of BOMF-based epoxy resins can be tailored to meet technical and safety requirements of downstream applications, representing a sustainable alternative to traditional systems containing DGEBA.
Related Topics
Concepts
Epoxy
Materials science
Thermosetting polymer
Maleic anhydride
Adhesive
Curing (chemistry)
Composite material
Dynamic mechanical analysis
Differential scanning calorimetry
Bisphenol A
Ultimate tensile strength
Glass transition
Diglycidyl ether
Polymer
Copolymer
Layer (electronics)
Thermodynamics
Physics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1007/s10853-023-08458-8
- https://link.springer.com/content/pdf/10.1007/s10853-023-08458-8.pdf
- OA Status
- hybrid
- Cited By
- 20
- References
- 54
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4366579972
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4366579972Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1007/s10853-023-08458-8Digital Object Identifier
- Title
-
Fully bio-based furan/maleic anhydride epoxy resin with enhanced adhesive propertiesWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
-
2023-04-01Full publication date if available
- Authors
-
Noemi Faggio, A. Marotta, Veronica Ambrogi, Pierfrancesco Cerruti, Gennaro GentileList of authors in order
- Landing page
-
https://doi.org/10.1007/s10853-023-08458-8Publisher landing page
- PDF URL
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https://link.springer.com/content/pdf/10.1007/s10853-023-08458-8.pdfDirect link to full text PDF
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
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https://link.springer.com/content/pdf/10.1007/s10853-023-08458-8.pdfDirect OA link when available
- Concepts
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Epoxy, Materials science, Thermosetting polymer, Maleic anhydride, Adhesive, Curing (chemistry), Composite material, Dynamic mechanical analysis, Differential scanning calorimetry, Bisphenol A, Ultimate tensile strength, Glass transition, Diglycidyl ether, Polymer, Copolymer, Layer (electronics), Thermodynamics, PhysicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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20Total citation count in OpenAlex
- Citations by year (recent)
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2025: 5, 2024: 13, 2023: 2Per-year citation counts (last 5 years)
- References (count)
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54Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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