Glass/steel/clay interactions in a simulated radioactive waste geological disposal system Article Swipe
István Tolnai
,
János Osán
,
Ottó Czömpöly
,
Attila Sulyok
,
Margit Fábián
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1038/s41598-023-47578-8
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1038/s41598-023-47578-8
Deep geological storage is the accepted solution for the final disposal of high-level radioactive waste therefore, it is necessary to study the host rock of the planned Hungarian waste repository and the materials involved in the engineered barriers. The main goal was to understand the characteristics and stability of the glass/steel/claystone system, from the structural properties of the vitrified waste (borosilicate glasses) to the clay response in the repository. Repository conditions were applied during the experiments to understand the chemical evolution of the system. A triplicate setup was kept at 80 °C for 3, 7 and 12 months and post-mortem characterization was performed. No alteration products were observed with scanning electron microscopy energy dispersive X-ray spectroscopy measurements on the surface of the glass and Fe or in the clay after the end of the experimental period. Based on the elemental analysis of the liquid phase, the released amount of B, K, Si and Na increased, while that of Ca and Mg decreased compared to the baseline. The concentrations of Cl − and SO 4 2− did not change significantly. Ca- and Mg-silicate precipitation was observed by X-ray photoelectron spectroscopy at the surface range of the borosilicate glasses because of the synthetic porewater treatment.
Related Topics
Concepts
Borosilicate glass
Radioactive waste
X-ray photoelectron spectroscopy
High-level waste
Materials science
Spent nuclear fuel
Scanning electron microscope
Precipitation
Waste disposal
Clay minerals
Chemical engineering
Mineralogy
Nuclear chemistry
Metallurgy
Waste management
Chemistry
Composite material
Engineering
Meteorology
Physics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41598-023-47578-8
- https://www.nature.com/articles/s41598-023-47578-8.pdf
- OA Status
- gold
- Cited By
- 4
- References
- 26
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4388854214
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4388854214Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1038/s41598-023-47578-8Digital Object Identifier
- Title
-
Glass/steel/clay interactions in a simulated radioactive waste geological disposal systemWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-11-21Full publication date if available
- Authors
-
István Tolnai, János Osán, Ottó Czömpöly, Attila Sulyok, Margit FábiánList of authors in order
- Landing page
-
https://doi.org/10.1038/s41598-023-47578-8Publisher landing page
- PDF URL
-
https://www.nature.com/articles/s41598-023-47578-8.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
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https://www.nature.com/articles/s41598-023-47578-8.pdfDirect OA link when available
- Concepts
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Borosilicate glass, Radioactive waste, X-ray photoelectron spectroscopy, High-level waste, Materials science, Spent nuclear fuel, Scanning electron microscope, Precipitation, Waste disposal, Clay minerals, Chemical engineering, Mineralogy, Nuclear chemistry, Metallurgy, Waste management, Chemistry, Composite material, Engineering, Meteorology, PhysicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
4Total citation count in OpenAlex
- Citations by year (recent)
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2025: 3, 2024: 1Per-year citation counts (last 5 years)
- References (count)
-
26Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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