Growth-Driven Polymorphism Engineering and Direct Phase Modulation of α- and β′-In2Se3 Article Swipe
Tianru Wu
,
Lei Xu
,
Dongyan Liu
,
Zhenhua Wu
,
Han Chen
,
Yutao Han
,
Mingzheng Wang
,
Haoyue Guo
,
Tian Tan
,
Yakui Mu
,
Yang Wang
,
Zhongchen Song
,
Qunli Rao
,
Xuewei Feng
,
Yakun Yuan
,
Lei Shi
,
Xiaotian Zhang
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-7385740/v1
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-7385740/v1
Two-dimensional (2D) In2Se3 represents a uniquely versatile platform for novel electronics, hosting the rare coexistence of paraelectric (β), antiferroelectric (β'), and ferroelectric (α) phases. However, synthesizing phase-pure In2Se3 films, particularly the critical ferroelectric semiconducting α-phase, is fundamentally hindered by the subtle structural distinctions and minimal energetic differences among its polymorphs. Here, we directly reveal phase-selective growth of In2Se3 on mica using cross-sectional transmission electron microscopy (TEM). It is found that both chemical vapor deposition (CVD) and physical vapor deposition (PVD) techniques yield exclusively either the pure β′ phase or coexisting monolayer α and β′ phases, with the cooling rate playing a critical role in phase selection. Crucially, in situ stress release within the epitaxial film on mica generates wrinkles propagating along the <> direction, triggering an immediate β' to α phase transformation. The resulting phase-pure α-In2Se3 films enable ferroelectric transistors exhibiting a high electron mobility of 259 cm2 V-1 s-1. This precise control over polymorph synthesis unlocks promising opportunities for 2D ferroelectric devices and nanoelectronics, offering a pathway to harness phase-specific functionalities.
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- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.21203/rs.3.rs-7385740/v1
- https://www.researchsquare.com/article/rs-7385740/latest.pdf
- OA Status
- gold
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4413795797
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Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4413795797Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.21203/rs.3.rs-7385740/v1Digital Object Identifier
- Title
-
Growth-Driven Polymorphism Engineering and Direct Phase Modulation of α- and β′-In2Se3Work title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-08-28Full publication date if available
- Authors
-
Tianru Wu, Lei Xu, Dongyan Liu, Zhenhua Wu, Han Chen, Yutao Han, Mingzheng Wang, Haoyue Guo, Tian Tan, Yakui Mu, Yang Wang, Zhongchen Song, Qunli Rao, Xuewei Feng, Yakun Yuan, Lei Shi, Xiaotian ZhangList of authors in order
- Landing page
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https://doi.org/10.21203/rs.3.rs-7385740/v1Publisher landing page
- PDF URL
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https://www.researchsquare.com/article/rs-7385740/latest.pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.researchsquare.com/article/rs-7385740/latest.pdfDirect OA link when available
- Concepts
-
Ferroelectricity, Materials science, Epitaxy, Phase (matter), Monolayer, Chemical vapor deposition, Transmission electron microscopy, Crystallography, Electron diffraction, Dielectric, Nanotechnology, Microelectronics, Optoelectronics, Chemistry, Diffraction, Layer (electronics), Optics, Physics, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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