High-Performance Lithium Sulfur Batteries Based on Multidimensional Graphene-CNT-Nanosulfur Hybrid Cathodes Article Swipe
Álvaro Doñoro
,
Álvaro Muñoz-Mauricio
,
Vinodkumar Etacheri
·
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.3390/batteries7020026
YOU?
·
· 2021
· Open Access
·
· DOI: https://doi.org/10.3390/batteries7020026
Although lithium-sulfur (Li-S) batteries are one of the promising candidates for next-generation energy storage, their practical implementation is limited by rapid capacity fading due to lithium polysulfide (LiPSs) formation and the low electronic conductivity of sulfur. Herein, we report a high-performance lithium-sulfur battery based on multidimensional cathode architecture consisting of nanosulfur, graphene nanoplatelets (2D) and multiwalled carbon nanotubes (1D). The ultrasonic synthesis method results in the generation of sulfur nanoparticles and their intercalation into the multilayered graphene nanoplatelets. The optimized multidimensional graphene-sulfur-CNT hybrid cathode (GNS58-CNT10) demonstrated a high specific capacity (1067 mAh g−1 @ 50 mA g−1), rate performance (539 @ 1 A g−1), coulombic efficiency (~95%) and cycling stability (726 mAh g−1 after 100 cycles @ 200 mA g−1) compared to the reference cathode. Superior electrochemical performances are credited to the encapsulation of nanosulfur between the individual layers of graphene nanoplatelets with high electronic conductivity, and effective polysulfide trapping by MWCNT bundles.
Related Topics
Concepts
Polysulfide
Graphene
Materials science
Faraday efficiency
Cathode
Sulfur
Lithium–sulfur battery
Carbon nanotube
Electrochemistry
Chemical engineering
Nanotechnology
Conductivity
Lithium (medication)
Battery (electricity)
Nanoparticle
Electrode
Chemistry
Endocrinology
Engineering
Physical chemistry
Metallurgy
Physics
Medicine
Quantum mechanics
Electrolyte
Power (physics)
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/batteries7020026
- https://www.mdpi.com/2313-0105/7/2/26/pdf?version=1618798614
- OA Status
- gold
- Cited By
- 23
- References
- 88
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W3152884464
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W3152884464Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.3390/batteries7020026Digital Object Identifier
- Title
-
High-Performance Lithium Sulfur Batteries Based on Multidimensional Graphene-CNT-Nanosulfur Hybrid CathodesWork title
- Type
-
articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2021Year of publication
- Publication date
-
2021-04-19Full publication date if available
- Authors
-
Álvaro Doñoro, Álvaro Muñoz-Mauricio, Vinodkumar EtacheriList of authors in order
- Landing page
-
https://doi.org/10.3390/batteries7020026Publisher landing page
- PDF URL
-
https://www.mdpi.com/2313-0105/7/2/26/pdf?version=1618798614Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
-
https://www.mdpi.com/2313-0105/7/2/26/pdf?version=1618798614Direct OA link when available
- Concepts
-
Polysulfide, Graphene, Materials science, Faraday efficiency, Cathode, Sulfur, Lithium–sulfur battery, Carbon nanotube, Electrochemistry, Chemical engineering, Nanotechnology, Conductivity, Lithium (medication), Battery (electricity), Nanoparticle, Electrode, Chemistry, Endocrinology, Engineering, Physical chemistry, Metallurgy, Physics, Medicine, Quantum mechanics, Electrolyte, Power (physics)Top concepts (fields/topics) attached by OpenAlex
- Cited by
-
23Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 4, 2024: 8, 2023: 2, 2022: 9Per-year citation counts (last 5 years)
- References (count)
-
88Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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