High-Performance Non-doped Blue OLEDs based on Efficiently Triplet-Triplet Upconversion and Aggregation-induced Emission Article Swipe
YOU?
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· 2021
· Open Access
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· DOI: https://doi.org/10.26434/chemrxiv.13550579.v1
Triplet-triplet upconversion (TTU), where two low-energy triplet excitons are converted to one higher energy singlet exciton, is excellent approach to break through the theoretical limit of the pure fluorescent organic light-emitting diodes (OLEDs) by 5%. To data, however, the reported emitters with high emission efficiency and efficiently TTU in film state are rare. Herein, we design the blue aggregation-induced emission luminogens (AIEgens) and investigate their upconversion efficiency. TPA-An-mPhCz can not only achieve high emission efficiency in the film state, but also show high upconversion efficiency of close to 50% even though the calculated energy level of the triplet excitons (T 2 ) is lower than 2T 1 . A possible upconversion mechanism is proposed according to the transient electroluminescence spectra and theoretical calculation. This strategy may provide a new platform for the construction of highly efficient non-doped blue OLEDs based on TTU and AIEgens.
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- preprint
- Language
- en
- Landing Page
- https://doi.org/10.26434/chemrxiv.13550579.v1
- OA Status
- gold
- Related Works
- 10
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- https://openalex.org/W3208271104
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https://openalex.org/W3208271104Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.26434/chemrxiv.13550579.v1Digital Object Identifier
- Title
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High-Performance Non-doped Blue OLEDs based on Efficiently Triplet-Triplet Upconversion and Aggregation-induced EmissionWork title
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2021Year of publication
- Publication date
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2021-01-20Full publication date if available
- Authors
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Pengbo Han, Chengwei Lin, Kaojin Wang, Yanping Qiu, Haozhong Wu, Dongge Ma, Anjun Qin, Ben Zhong TangList of authors in order
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https://doi.org/10.26434/chemrxiv.13550579.v1Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
- OA URL
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https://doi.org/10.26434/chemrxiv.13550579.v1Direct OA link when available
- Concepts
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Photon upconversion, OLED, Optoelectronics, Exciton, Materials science, Electroluminescence, Doping, Singlet state, Triplet state, Diode, Photochemistry, Chemistry, Nanotechnology, Physics, Atomic physics, Molecule, Excited state, Condensed matter physics, Organic chemistry, Layer (electronics)Top concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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