High plating currents without dendrites at the interface between a lithium anode and solid electrolyte Article Swipe
Dominic L. R. Melvin
,
Marco Siniscalchi
,
Dominic Spencer Jolly
,
Bingkun Hu
,
Ziyang Ning
,
Shengming Zhang
,
Junfu Bu
,
Shashidhara Marathe
,
Anne Bonnin
,
Johannes Ihli
,
Gregory J. Rees
,
Patrick S. Grant
,
Charles W. Monroe
,
T.J. Marrow
,
Guanchen Li
,
Peter G. Bruce
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41560-025-01847-0
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41560-025-01847-0
Avoiding lithium dendrites at the lithium/ceramic electrolyte interface and, as a result, avoiding cell short circuit when plating at practical current densities remains a significant challenge for all-solid-state batteries. Typically, values are limited to around 1 mA cm −2 , even, for example, for garnets with a relative density of >99%. It is not obvious that simply densifying ceramic electrolytes will deliver high plating currents. Here we show that plating currents of 9 mA cm −2 can be achieved without dendrite formation, by densifying argyrodite, Li 6 PS 5 Cl, to 99%. Changes in the microstructure of Li 6 PS 5 Cl on densification from 83 to 99% were determined by focused ion beam-scanning electron microscopy tomography and used to calculate their effect on the critical current density (CCD). Modelling shows that not all changes in microstructure with densification act to increase CCD. Whereas smaller pores and shorter cracks increase CCD, lower pore population and narrower cracks act to decrease CCD. Calculations show that the former changes dominate over the latter, predicating an overall increase in CCD, as observed experimentally.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41560-025-01847-0
- https://www.nature.com/articles/s41560-025-01847-0.pdf
- OA Status
- hybrid
- Cited By
- 2
- References
- 79
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4413993000
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4413993000Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41560-025-01847-0Digital Object Identifier
- Title
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High plating currents without dendrites at the interface between a lithium anode and solid electrolyteWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-09-04Full publication date if available
- Authors
-
Dominic L. R. Melvin, Marco Siniscalchi, Dominic Spencer Jolly, Bingkun Hu, Ziyang Ning, Shengming Zhang, Junfu Bu, Shashidhara Marathe, Anne Bonnin, Johannes Ihli, Gregory J. Rees, Patrick S. Grant, Charles W. Monroe, T.J. Marrow, Guanchen Li, Peter G. BruceList of authors in order
- Landing page
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https://doi.org/10.1038/s41560-025-01847-0Publisher landing page
- PDF URL
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https://www.nature.com/articles/s41560-025-01847-0.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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hybridOpen access status per OpenAlex
- OA URL
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https://www.nature.com/articles/s41560-025-01847-0.pdfDirect OA link when available
- Concepts
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Anode, Electrolyte, Materials science, Plating (geology), Lithium metal, Lithium (medication), Chemical engineering, Metallurgy, Chemistry, Electrode, Medicine, Internal medicine, Physics, Engineering, Physical chemistry, GeophysicsTop concepts (fields/topics) attached by OpenAlex
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2Total citation count in OpenAlex
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2025: 2Per-year citation counts (last 5 years)
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79Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| cited_by_percentile_year.max | 97 |
| cited_by_percentile_year.min | 95 |
| corresponding_author_ids | https://openalex.org/A5056496930, https://openalex.org/A5084382073 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 16 |
| corresponding_institution_ids | https://openalex.org/I40120149, https://openalex.org/I7882870 |
| citation_normalized_percentile.value | 0.90662985 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |