High radiation tolerance of electrocaloric (1-x)Pb(Mg1/3Nb2/3)O3–xPbTiO3 Article Swipe
Hana Uršič
,
Uroš Prah
,
Tadej Rojac
,
Anže Jazbec
,
Luka Snoj
,
Silvo Drnovšek
,
Andraž Bradeško
,
Anja Mirjanić
,
Marko Vrabelj
,
Barbara Malič
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1016/j.jeurceramsoc.2022.05.051
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.1016/j.jeurceramsoc.2022.05.051
High radiation tolerance of functional materials in harsh environments is the key requirement for the operation of particle accelerators, medical devices, nuclear power plants, satellites, and spacecraft. Neutron and gamma (γ) radiation can seriously affect the functional properties of the irradiated materials and thus the performance of the entire device. In this work, the feasibility of using (1-x)Pb(Mg1/3Nb2/3)O3–xPbTiO3 (PMN–100xPT) electrocaloric materials in applications where the material is exposed to high neutron and γ-radiation is investigated. For this purpose, three different compositions of PMN–100xPT ceramics (x = 0, 0.1, and 0.35) were prepared and their dielectric, ferroelectric and electrocaloric properties were investigated before and after neutron and γ-irradiation. The samples were irradiated with a neutron fluence of 1015 to 1017 neutrons cm−2 with an energy of 1 MeV, which exceeds the largest expected neutron irradiation in the European Council for nuclear Research (CERN) and simultaneously exposed to γ-irradiation. The neutron and γ-radiation partially affect the functional properties of the PMN–35PT, the ceramic with distinct ferroelectric and weakened relaxor features, with some differences observed in the domain switching behavior, measured by conventional polarization versus electric field (P–E) hysteresis, at the highest radiation dose of 1017 neutrons cm−2. In contrast, the functional properties of the irradiated PMN and PMN–10PT samples with relaxor behavior are quite similar to those of the pristine samples, therefore, we conclude that these materials can be used as working materials in EC coolers exposed to such harsh environments.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.jeurceramsoc.2022.05.051
- OA Status
- hybrid
- Cited By
- 8
- References
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- Related Works
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- OpenAlex ID
- https://openalex.org/W4281480665
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4281480665Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.jeurceramsoc.2022.05.051Digital Object Identifier
- Title
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High radiation tolerance of electrocaloric (1-x)Pb(Mg1/3Nb2/3)O3–xPbTiO3Work title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2022Year of publication
- Publication date
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2022-05-25Full publication date if available
- Authors
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Hana Uršič, Uroš Prah, Tadej Rojac, Anže Jazbec, Luka Snoj, Silvo Drnovšek, Andraž Bradeško, Anja Mirjanić, Marko Vrabelj, Barbara MaličList of authors in order
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https://doi.org/10.1016/j.jeurceramsoc.2022.05.051Publisher landing page
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://doi.org/10.1016/j.jeurceramsoc.2022.05.051Direct OA link when available
- Concepts
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Materials science, Neutron, Irradiation, Ceramic, Radiation, Ferroelectricity, Fluence, Dielectric, Optoelectronics, Composite material, Nuclear physics, PhysicsTop concepts (fields/topics) attached by OpenAlex
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8Total citation count in OpenAlex
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2025: 3, 2024: 2, 2023: 3Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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