High-throughput exploration of structural and functional properties of the high entropy nitride system (Ti-Co-Mo-Ta-W)N Article Swipe
Ellen Suhr
,
Olga A. Krysiak
,
Valerie Strotkoetter
,
Wolfgang Schuhmann
,
Alfred Ludwig
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-1971704/v1
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.21203/rs.3.rs-1971704/v1
High entropy nitrides are largely unexplored materials with high potential to show good mechanical properties, high stability against chemicals, but also promising catalytic properties. The latter is due to their good electrical conductivity compared to (high entropy) oxides. The high entropy nitride system (Ti-Co-Mo-Ta-W)N was investigated, to combine binary and ternary nitrides, which show good water splitting activities. Continuous composition spread thin film materials libraries were deposited using reactive co-sputter deposition at 300 and 500°C. X-ray diffraction results show that the films consist of a single-phase solid solution in NaCl-type structure. The surface morphology, examined using scanning electron and atomic force microscopy, is related to the deposition temperature. (TiCoMoTaW)N films show low resistivity values in the range from 1.72 to 5.2 µΩ*cm. Their oxygen evolution reaction activity was measured using a scanning droplet cell, with a maximum current density of 1.78 \(\frac{\text{m}\text{A}}{{\text{c}\text{m}}^{2}}\) at 1700 mV vs. RHE at a Co-rich area. However, the stability under electrochemical load is critical.
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- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.21203/rs.3.rs-1971704/v1
- https://www.researchsquare.com/article/rs-1971704/latest.pdf
- OA Status
- green
- References
- 39
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4293582196
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4293582196Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.21203/rs.3.rs-1971704/v1Digital Object Identifier
- Title
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High-throughput exploration of structural and functional properties of the high entropy nitride system (Ti-Co-Mo-Ta-W)NWork title
- Type
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preprintOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2022Year of publication
- Publication date
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2022-08-30Full publication date if available
- Authors
-
Ellen Suhr, Olga A. Krysiak, Valerie Strotkoetter, Wolfgang Schuhmann, Alfred LudwigList of authors in order
- Landing page
-
https://doi.org/10.21203/rs.3.rs-1971704/v1Publisher landing page
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https://www.researchsquare.com/article/rs-1971704/latest.pdfDirect link to full text PDF
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YesWhether a free full text is available
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-
greenOpen access status per OpenAlex
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https://www.researchsquare.com/article/rs-1971704/latest.pdfDirect OA link when available
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Nitride, Throughput, High entropy alloys, Materials science, Nanotechnology, Computer science, Metallurgy, Microstructure, Operating system, Layer (electronics), WirelessTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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39Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.500°C. | 75 |
| abstract_inverted_index.Co-rich | 150 |
| abstract_inverted_index.against | 18 |
| abstract_inverted_index.combine | 48 |
| abstract_inverted_index.consist | 83 |
| abstract_inverted_index.current | 138 |
| abstract_inverted_index.density | 139 |
| abstract_inverted_index.droplet | 133 |
| abstract_inverted_index.entropy | 2, 41 |
| abstract_inverted_index.largely | 5 |
| abstract_inverted_index.maximum | 137 |
| abstract_inverted_index.nitride | 42 |
| abstract_inverted_index.oxides. | 38 |
| abstract_inverted_index.related | 104 |
| abstract_inverted_index.results | 78 |
| abstract_inverted_index.surface | 93 |
| abstract_inverted_index.ternary | 51 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.However, | 152 |
| abstract_inverted_index.activity | 127 |
| abstract_inverted_index.compared | 34 |
| abstract_inverted_index.electron | 98 |
| abstract_inverted_index.entropy) | 37 |
| abstract_inverted_index.examined | 95 |
| abstract_inverted_index.measured | 129 |
| abstract_inverted_index.nitrides | 3 |
| abstract_inverted_index.reaction | 126 |
| abstract_inverted_index.reactive | 69 |
| abstract_inverted_index.scanning | 97, 132 |
| abstract_inverted_index.solution | 88 |
| abstract_inverted_index.NaCl-type | 90 |
| abstract_inverted_index.catalytic | 23 |
| abstract_inverted_index.critical. | 159 |
| abstract_inverted_index.deposited | 67 |
| abstract_inverted_index.evolution | 125 |
| abstract_inverted_index.libraries | 65 |
| abstract_inverted_index.materials | 7, 64 |
| abstract_inverted_index.nitrides, | 52 |
| abstract_inverted_index.potential | 10 |
| abstract_inverted_index.promising | 22 |
| abstract_inverted_index.splitting | 57 |
| abstract_inverted_index.stability | 17, 154 |
| abstract_inverted_index.µΩ*cm. | 122 |
| abstract_inverted_index.Continuous | 59 |
| abstract_inverted_index.chemicals, | 19 |
| abstract_inverted_index.co-sputter | 70 |
| abstract_inverted_index.deposition | 71, 107 |
| abstract_inverted_index.electrical | 32 |
| abstract_inverted_index.mechanical | 14 |
| abstract_inverted_index.structure. | 91 |
| abstract_inverted_index.unexplored | 6 |
| abstract_inverted_index.activities. | 58 |
| abstract_inverted_index.composition | 60 |
| abstract_inverted_index.diffraction | 77 |
| abstract_inverted_index.microscopy, | 102 |
| abstract_inverted_index.morphology, | 94 |
| abstract_inverted_index.properties, | 15 |
| abstract_inverted_index.properties. | 24 |
| abstract_inverted_index.resistivity | 113 |
| abstract_inverted_index.(TiCoMoTaW)N | 109 |
| abstract_inverted_index.conductivity | 33 |
| abstract_inverted_index.single-phase | 86 |
| abstract_inverted_index.temperature. | 108 |
| abstract_inverted_index.investigated, | 46 |
| abstract_inverted_index.electrochemical | 156 |
| abstract_inverted_index.(Ti-Co-Mo-Ta-W)N | 44 |
| abstract_inverted_index.\(\frac{\text{m}\text{A}}{{\text{c}\text{m}}^{2}}\) | 142 |
| cited_by_percentile_year | |
| countries_distinct_count | 1 |
| institutions_distinct_count | 5 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/6 |
| sustainable_development_goals[0].score | 0.7699999809265137 |
| sustainable_development_goals[0].display_name | Clean water and sanitation |
| citation_normalized_percentile.value | 0.10916244 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |