Highly efficient hydrodesulfurization driven by an in-situ reconstruction of ammonium/amine intercalated MoS2 catalysts Article Swipe
Tianlan Yan
,
Yingshuai Jia
,
Kaige Hou
,
Zhuxin Gui
,
Wenbiao Zhang
,
Ke Du
,
Di Pan
,
He Li
,
Yanghao Shi
,
Lu Qi
,
Qingsheng Gao
,
Yahong Zhang
,
Yi Tang
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1016/j.isci.2024.109824
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1016/j.isci.2024.109824
Hydrodesulfurization (HDS) is a commonly used route for producing clean fuels in modern refinery. Herein, ammonium/amine-intercalated MoS2 catalysts with various content of 1T phase and S vacancies have been successfully synthesized. Along with the increment of 1T phase and S vacancies of MoS2, the initial reaction rate of the HDS of dibenzothiophene (DBT) can be improved from 0.09 to 0.55 μmol·gcat-1·s-1, accounting for a remarkable activity compared to the-state-of-the-art catalysts. In a combinatory study via the activity evaluation and catalysts characterization, we found that the intercalation species of MoS2 played a key role in generating more 1T phase and S vacancies through the 'intercalation-deintercalation' processes, and the hydrogenation and desulfurization of HDS can be significantly promoted by 1T phase and S vacancies on MoS2, respectively. This study provides a practically meaningful guidance for developing more advanced HDS catalysts by the intercalated MoS2-derived materials with an in-depth understanding of structure-function relationships.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.isci.2024.109824
- OA Status
- gold
- Cited By
- 8
- References
- 64
- Related Works
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- OpenAlex ID
- https://openalex.org/W4395663089
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4395663089Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.isci.2024.109824Digital Object Identifier
- Title
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Highly efficient hydrodesulfurization driven by an in-situ reconstruction of ammonium/amine intercalated MoS2 catalystsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
-
2024Year of publication
- Publication date
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2024-04-26Full publication date if available
- Authors
-
Tianlan Yan, Yingshuai Jia, Kaige Hou, Zhuxin Gui, Wenbiao Zhang, Ke Du, Di Pan, He Li, Yanghao Shi, Lu Qi, Qingsheng Gao, Yahong Zhang, Yi TangList of authors in order
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https://doi.org/10.1016/j.isci.2024.109824Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://doi.org/10.1016/j.isci.2024.109824Direct OA link when available
- Concepts
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Hydrodesulfurization, Amine gas treating, Catalysis, Ammonium, Refinery, Chemistry, In situ, Inorganic chemistry, Materials science, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
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8Total citation count in OpenAlex
- Citations by year (recent)
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2025: 6, 2024: 2Per-year citation counts (last 5 years)
- References (count)
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64Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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