Highly Linearized Twisted Iridium(III) Complexes Article Swipe

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Ross J. Davidson , Yu‐Ting Hsu , Gareth C. Griffiths , Chenfei Li , Dmitry S. Yufit , Róbert Pál , Andrew Beeby ·

YOU? · · 2018 · Open Access · · DOI: https://doi.org/10.1021/acs.inorgchem.8b02818

Improving the spatial alignment of emitting molecules has long been a goal of organic-light-emitting-diode development to improve device efficiencies and to generate polarized emission. Herein we describe a simple approach employing Sonogashira coupling with alkyne iridium(phenylpyridine)₂(acetylacetone) synthons (2-5) to generate eight linear iridium complexes (6-13) with crystallographically determined lengths of up to 5 nm. By embedding these "long" complexes into a polymer matrix and stretching it, an improvement of the polarization ratio of unstretched and stretched films of up to 7.1 times was achieved. Additionally, through the inclusion of "twists" in the complexes, the electronic coupling between the iridium center and substituent was controlled, giving a system where the emission behavior is independent of the length.

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Chemistry Iridium Crystallography Computational chemistry Stereochemistry Organic chemistry Catalysis

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Type: article
Language: en
Landing Page: https://doi.org/10.1021/acs.inorgchem.8b02818
OA Status: gold
Cited By: 8
References: 33
Related Works: 10
OpenAlex ID: https://openalex.org/W2899261113

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DOI: https://doi.org/10.1021/acs.inorgchem.8b02818

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Title: Highly Linearized Twisted Iridium(III) Complexes

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Language: en

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Publication year: 2018

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Publication date: 2018-11-01

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Authors: Ross J. Davidson, Yu‐Ting Hsu, Gareth C. Griffiths, Chenfei Li, Dmitry S. Yufit, Róbert Pál, Andrew Beeby

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Landing page: https://doi.org/10.1021/acs.inorgchem.8b02818

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OA status: gold

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Concepts: Chemistry, Iridium, Crystallography, Computational chemistry, Stereochemistry, Organic chemistry, Catalysis

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Cited by: 8

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