Highly Responsive Polar Vortices in All‐Ferroelectric Heterostructures Article Swipe
Pravin Kavle
,
Aiden Ross
,
Harikrishnan KP
,
Peter Meisenheimer
,
Arvind Dasgupta
,
Jiyuan Yang
,
Ching‐Che Lin
,
Hao Pan
,
Piush Behera
,
Eric Parsonnet
,
Xiaoxi Huang
,
Jacob A. Zorn
,
Yu‐Tsun Shao
,
Sujit Das
,
Shi Liu
,
David A. Muller
,
R. Ramesh
,
Long‐Qing Chen
,
Lane W. Martin
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202410146
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202410146
The discovery of polar vortices and skyrmions in ferroelectric‐dielectric superlattices [such as (PbTiO 3 ) n /(SrTiO 3 ) n ] has ushered in an era of novel dipolar topologies and corresponding emergent phenomena. The key to creating such emergent features has generally been considered to be related to counterpoising strongly polar and non‐polar materials thus creating the appropriate boundary conditions. This limits the utility these materials can have, however, by rendering (effectively) half of the structure unresponsive to applied stimuli. Here, using advanced thin‐film deposition and an array of characterization and simulation approaches, polar vortices are realized in all‐ferroelectric trilayers, multilayers, and superlattices built from the fundamental building block of (PbTiO 3 ) n /(Pb x Sr 1− x TiO 3 ) n wherein in‐plane ferroelectric polarization in the Pb x Sr 1− x TiO 3 provides the appropriate boundary conditions. These superlattices exhibit substantially enhanced electromechanical and ferroelectric responses in the out‐of‐plane direction that arise from the ability of the polarization in both layers to rotate to the out‐of‐plane direction under field. In the in‐plane direction, the layers are found to be strongly coupled during switching and when heterostructured with ferroelectric‐dielectric building blocks, it is possible to produce multistate switching. This approach expands the realm of systems supporting emergent dipolar texture formation and does so with entirely ferroelectric materials thus greatly improving their responses.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/adma.202410146
- OA Status
- green
- Cited By
- 4
- References
- 46
- Related Works
- 10
- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4404322799Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/adma.202410146Digital Object Identifier
- Title
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Highly Responsive Polar Vortices in All‐Ferroelectric HeterostructuresWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-11-13Full publication date if available
- Authors
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Pravin Kavle, Aiden Ross, Harikrishnan KP, Peter Meisenheimer, Arvind Dasgupta, Jiyuan Yang, Ching‐Che Lin, Hao Pan, Piush Behera, Eric Parsonnet, Xiaoxi Huang, Jacob A. Zorn, Yu‐Tsun Shao, Sujit Das, Shi Liu, David A. Muller, R. Ramesh, Long‐Qing Chen, Lane W. MartinList of authors in order
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https://doi.org/10.1002/adma.202410146Publisher landing page
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YesWhether a free full text is available
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/2503974Direct OA link when available
- Concepts
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Materials science, Polar, Ferroelectricity, Heterojunction, Vortex, Polar vortex, Nanotechnology, Optoelectronics, Condensed matter physics, Dielectric, Meteorology, Astronomy, PhysicsTop concepts (fields/topics) attached by OpenAlex
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4Total citation count in OpenAlex
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2025: 3, 2024: 1Per-year citation counts (last 5 years)
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46Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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