Host–guest complexation‐induced chirality switching of pillararenes by perylene diimide‐based hexagonal metallacages Article Swipe
Yali Hou
,
Chaoqun Mu
,
Yunzhi Shi
,
Zeyuan Zhang
,
Haifei Liu
,
Zilin Zhou
,
Sanliang Ling
,
Bingbing Shi
,
Xianglong Duan
,
Cheng Yang
,
Mingming Zhang
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/agt2.628
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/agt2.628
Chirality in confined nanospaces has brought some new insights into chirality transfer, amplification, and chiroptical properties. However, chirality switching, which is a common phenomenon in biological systems, has never been realized in confined environments. Herein, we report a type of hexagonal metallacages that shows good host–guest interactions with ethoxy pillar[5]arene and pillar[6]arene, as confirmed by single‐crystal X‐ray analysis. Importantly, when a chiral pillar[5]arene‐based molecular universal joint (MUJ) is used as the guest, the host–guest complexation would drive the alkyl ring of the MUJ flip from outside to inside the cavity of its pillar[5]arene unit, which enables the configuration change along with the chirality inversion of the MUJ. Moreover, the host–guest complexation facilitates the chirality transfer from guests to hosts, giving circularly polarized luminescence to the system. This study provides a unique metallacage‐pillararene recognition motif for the chirality switching of planar chiral pillararenes, which will promote the construction of host–guest systems with tunable chirality for advanced applications.
Related Topics
Concepts
Chirality (physics)
Supramolecular chirality
Perylene
Pillar
Diimide
Planar chirality
Crystallography
Chemistry
Supramolecular chemistry
Materials science
Nanotechnology
Crystal structure
Molecule
Enantioselective synthesis
Physics
Organic chemistry
Quantum mechanics
Nambu–Jona-Lasinio model
Quark
Engineering
Chiral symmetry breaking
Catalysis
Structural engineering
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/agt2.628
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/agt2.628
- OA Status
- gold
- Cited By
- 17
- References
- 56
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4400136073
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4400136073Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1002/agt2.628Digital Object Identifier
- Title
-
Host–guest complexation‐induced chirality switching of pillararenes by perylene diimide‐based hexagonal metallacagesWork title
- Type
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articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-06-27Full publication date if available
- Authors
-
Yali Hou, Chaoqun Mu, Yunzhi Shi, Zeyuan Zhang, Haifei Liu, Zilin Zhou, Sanliang Ling, Bingbing Shi, Xianglong Duan, Cheng Yang, Mingming ZhangList of authors in order
- Landing page
-
https://doi.org/10.1002/agt2.628Publisher landing page
- PDF URL
-
https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/agt2.628Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
-
https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/agt2.628Direct OA link when available
- Concepts
-
Chirality (physics), Supramolecular chirality, Perylene, Pillar, Diimide, Planar chirality, Crystallography, Chemistry, Supramolecular chemistry, Materials science, Nanotechnology, Crystal structure, Molecule, Enantioselective synthesis, Physics, Organic chemistry, Quantum mechanics, Nambu–Jona-Lasinio model, Quark, Engineering, Chiral symmetry breaking, Catalysis, Structural engineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
17Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 14, 2024: 3Per-year citation counts (last 5 years)
- References (count)
-
56Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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