How horizontal transport and turbulent mixing impact aerosol particle and precursor concentrations at a background site in the UAE Article Swipe
Jutta Kesti
,
Ewan O’Connor
,
Anne Hirsikko
,
John Backman
,
Maria Filioglou
,
Anu‐Maija Sundström
,
Juha Tonttila
,
Heikki Lihavainen
,
Hannele Korhonen
,
Eija Asmi
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.5194/acp-24-9369-2024
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.5194/acp-24-9369-2024
The optical, physical, and chemical properties of aerosol particles have been previously studied in the United Arab Emirates (UAE), but there is still a gap in the knowledge of particle sources and in the horizontal and vertical transport of aerosol particles and their precursors in the area. To investigate how aerosol particle and SO2 concentrations at the surface responded to changes in horizontal and vertical transport, we used data from a 1-year measurement campaign at a background site where local sources of SO2 were expected to be minimal. The measurement campaign provided a combination of in situ measurements at the surface and the boundary layer evolution from vertical and horizontal wind profiles measured by a Doppler lidar. The diurnal structure of the boundary layer in the UAE was very similar from day to day, with a deep, well-mixed boundary layer during the day transitioning to a shallow nocturnal layer, with the maximum boundary layer height usually being reached around 14:00 local time. Both SO2 and nucleation-mode aerosol particle concentrations were elevated for surface winds coming from the east or western sectors. We attribute this to oil refineries located on the eastern and western coasts of the UAE. The concentrations of larger cloud condensation nuclei (CCN)-sized particles and their activation fraction did not show any clear dependence on wind direction, but the CCN number concentration showed some dependence on wind speed, with higher concentrations coinciding with the weakest surface winds. Peaks in SO2 concentrations were also observed despite low surface wind speeds and wind directions unfavourable for transport. However, winds aloft were much stronger, with wind speeds of 10 m s−1 at 1 km common at night and wind directions favourable for transport; surface-measured concentrations increased rapidly once these particular layers started to be entrained into the growing boundary layer, even if the surface wind direction was from a clean sector. These conditions also displayed higher nucleation-mode aerosol particle concentrations, i.e. new particle formation events occurring due to the increase in the gaseous precursor.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.5194/acp-24-9369-2024
- OA Status
- gold
- Cited By
- 1
- References
- 46
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- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4401963089Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.5194/acp-24-9369-2024Digital Object Identifier
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How horizontal transport and turbulent mixing impact aerosol particle and precursor concentrations at a background site in the UAEWork title
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articleOpenAlex work type
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enPrimary language
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2024Year of publication
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2024-08-28Full publication date if available
- Authors
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Jutta Kesti, Ewan O’Connor, Anne Hirsikko, John Backman, Maria Filioglou, Anu‐Maija Sundström, Juha Tonttila, Heikki Lihavainen, Hannele Korhonen, Eija AsmiList of authors in order
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https://doi.org/10.5194/acp-24-9369-2024Publisher landing page
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goldOpen access status per OpenAlex
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https://doi.org/10.5194/acp-24-9369-2024Direct OA link when available
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Aerosol, Turbulence, Mixing (physics), Environmental science, Atmospheric sciences, Particle (ecology), Vertical mixing, Meteorology, Mechanics, Physics, Geology, Oceanography, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
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1Total citation count in OpenAlex
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2024: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W4248382853, https://openalex.org/W3160538308, https://openalex.org/W3190614793, https://openalex.org/W2064943738, https://openalex.org/W2888746173, https://openalex.org/W2560228938, https://openalex.org/W2143093706, https://openalex.org/W3184345837, https://openalex.org/W1975871536, https://openalex.org/W4253740333, https://openalex.org/W4312938581, https://openalex.org/W2586906818, https://openalex.org/W2016932556, https://openalex.org/W3011899476, https://openalex.org/W2917309512, https://openalex.org/W2005096647, https://openalex.org/W4226077659, https://openalex.org/W4401963089, https://openalex.org/W2044284750, https://openalex.org/W1639761881, https://openalex.org/W2012165084, https://openalex.org/W1544276658, https://openalex.org/W2117004231, https://openalex.org/W1053885566, https://openalex.org/W2044933586, https://openalex.org/W2326623930, https://openalex.org/W2811505569, https://openalex.org/W2090687131, https://openalex.org/W2127722963, https://openalex.org/W2941596473, https://openalex.org/W2167088427, https://openalex.org/W1998160649, https://openalex.org/W1844239817, https://openalex.org/W2011254556, https://openalex.org/W1485504984, https://openalex.org/W1975964212, https://openalex.org/W2127781078, https://openalex.org/W4312384569, https://openalex.org/W3119370400, https://openalex.org/W2614613011, https://openalex.org/W2792076794, https://openalex.org/W3156447188, https://openalex.org/W2111570465, https://openalex.org/W2073933662, https://openalex.org/W2074626375, https://openalex.org/W4313897305 |
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