How non-equilibrium aerosol chemistry impacts particle acidity: the GMXe AERosol CHEMistry (GMXe–AERCHEM, v1.0) sub-submodel of MESSy Article Swipe
Simon Rosanka
,
Holger Tost
,
Rolf Sander
,
Patrick Jöckel
,
Astrid Kerkweg
,
Domenico Taraborrelli
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.5194/egusphere-2023-2587
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.5194/egusphere-2023-2587
Aqueous-phase chemical processes in clouds, fog, and deliquescent aerosols are known to alter atmospheric composition and acidity significantly. Traditionally, global and regional models predict aerosol composition by relying on thermodynamic equilibrium models and neglect non-equilibrium processes. Here, we present the AERosol CHEMistry (GMXe–AERCHEM, v1.0) sub-submodel developed for the Modular Earth Submodel System (MESSy) as an add-on to the thermodynamic equilibrium model (i.e., ISORROPIA-II) used by MESSy’s Global Modal-aerosol eXtension (GMXe) submodel. AERCHEM allows the representation of non-equilibrium aqueous-phase chemistry of varying complexity in deliquescent fine aerosols. We perform a global simulation for the year 2010 by using the available detailed kinetic model for the chemistry of inorganic and small oxygenated organics. We evaluate AERCHEM’s performance by comparing the simulated concentrations of sulfate, nitrate, ammonium, and chloride to in situ measurements of three monitoring networks. Overall, AERCHEM reproduces observed concentrations reasonably well. We find that especially in the USA, the consideration of non-equilibrium chemistry in deliquescent aerosols reduces the model bias for sulfate, nitrate, and ammonium, when compared to simulated concentrations by ISORROPIA-II. Over most continental regions, fine aerosol acidity simulated by AERCHEM is similar to the predictions by ISORROPIA-II but tends to simulate slightly lower aerosol acidity in most regions. The consideration of non-equilibrium chemistry in deliquescent aerosols leads to a significant higher aerosol acidity in the marine boundary layer, which is in line with observations and recent literature. AERCHEM allows investigating the global-scale impact of aerosol non-equilibrium chemistry on atmospheric composition. This will aid the exploration of key multiphase processes and improve the model predictions for oxidation capacity and aerosols in the troposphere.
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- Type
- preprint
- Language
- en
- Landing Page
- https://doi.org/10.5194/egusphere-2023-2587
- OA Status
- gold
- Cited By
- 2
- References
- 15
- Related Works
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- OpenAlex ID
- https://openalex.org/W4388701655
All OpenAlex metadata
Raw OpenAlex JSON
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https://doi.org/10.5194/egusphere-2023-2587Digital Object Identifier
- Title
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How non-equilibrium aerosol chemistry impacts particle acidity: the GMXe AERosol CHEMistry (GMXe–AERCHEM, v1.0) sub-submodel of MESSyWork title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-11-15Full publication date if available
- Authors
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Simon Rosanka, Holger Tost, Rolf Sander, Patrick Jöckel, Astrid Kerkweg, Domenico TaraborrelliList of authors in order
- Landing page
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https://doi.org/10.5194/egusphere-2023-2587Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://doi.org/10.5194/egusphere-2023-2587Direct OA link when available
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Aerosol, Chemistry, Sulfate, Thermodynamic equilibrium, Chemical equilibrium, Nitrate, Aqueous solution, Environmental chemistry, Thermodynamics, Physical chemistry, Organic chemistry, PhysicsTop concepts (fields/topics) attached by OpenAlex
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2Total citation count in OpenAlex
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2024: 2Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W2055490230, https://openalex.org/W4393785072, https://openalex.org/W1568287675, https://openalex.org/W3083289182, https://openalex.org/W1936252359, https://openalex.org/W4293485763, https://openalex.org/W2032072526, https://openalex.org/W2079404410, https://openalex.org/W4231380648, https://openalex.org/W3113107862, https://openalex.org/W2013673272, https://openalex.org/W3114684333, https://openalex.org/W4385191539, https://openalex.org/W4256592402, https://openalex.org/W2893902463 |
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| corresponding_author_ids | https://openalex.org/A5091649637, https://openalex.org/A5043977638, https://openalex.org/A5012769954, https://openalex.org/A5090309042, https://openalex.org/A5040485527, https://openalex.org/A5007931712 |
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| institutions_distinct_count | 6 |
| corresponding_institution_ids | https://openalex.org/I171892758, https://openalex.org/I197323543, https://openalex.org/I204250578, https://openalex.org/I2898391981, https://openalex.org/I4210113422 |
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| sustainable_development_goals[0].display_name | Life below water |
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