Humidity-controlled interactions and lifting of MoS₂ on SiO₂ Article Swipe

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Sebastiaan Haartsen , Jantinus Wisman , Harold J. W. Zandvliet , Pantelis Bampoulis ·

YOU? · · 2025 · Open Access · · DOI: https://doi.org/10.1088/2515-7639/adaaa1

Fabrication of 2D material devices under ambient conditions faces challenges from humidity-dependent interfacial interactions and doping effects due to intercalated water layers. This study explores adhesion and force dynamics for a monolayer of molybdenum disulfide (MoS 2 ) on silicon dioxide (SiO 2 ) as a function of humidity, using atomic force microscopy (AFM). At low humidity (<10%RH), capillary forces dominate due to a liquid bridge forming between the AFM tip and sample. At intermediate humidity 40%RH, an additional water layer intercalates between the MoS 2 and the SiO 2 and the capillary force model alone is insufficient to describe the tip-sample interactions. Force-distance spectroscopy reveals additional force dynamics related to MoS 2 -lifting and dynamics in the intercalated water. Above 60%RH, water condenses on the MoS 2 and the capillary interactions are reduced. Understanding and identifying these interactions is crucial for optimising deposition of 2D materials under humid conditions.

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Humidity

Environmental Science

Materials Science

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Humidity Environmental science Materials science Atmospheric sciences Meteorology Geology Physics

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Type: article
Language: en
Landing Page: https://doi.org/10.1088/2515-7639/adaaa1
OA Status: gold
References: 54
Related Works: 10
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DOI: https://doi.org/10.1088/2515-7639/adaaa1

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Title: Humidity-controlled interactions and lifting of MoS₂ on SiO₂

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Type: article

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Language: en

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Publication year: 2025

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Publication date: 2025-01-15

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Authors: Sebastiaan Haartsen, Jantinus Wisman, Harold J. W. Zandvliet, Pantelis Bampoulis

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Landing page: https://doi.org/10.1088/2515-7639/adaaa1

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OA status: gold

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OA URL: https://doi.org/10.1088/2515-7639/adaaa1

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Concepts: Humidity, Environmental science, Materials science, Atmospheric sciences, Meteorology, Geology, Physics

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Humidity-controlled interactions and lifting of MoS2 on SiO2 Article Swipe

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Humidity-controlled interactions and lifting of MoS₂ on SiO₂ Article Swipe