Hydrogen sensing with high-performance via O- ion spillover at Pd single atoms stabilized SnO2 interface Article Swipe
Yinyin Qian
,
Guorui Zhao
,
Changming Zhang
,
Shengjie Yin
,
Junwei Chen
,
Yuanyuan Luo
,
Zhengfeng Huang
,
Bo Liu
,
Guotao Duan
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s43246-025-00865-5
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s43246-025-00865-5
Developing hydrogen sensors with high performances is imperative for facilitating H2-related industries. Metal oxide semiconductor (MOS) based gas sensors are simple structures with low cost that are a promising approach for H2 detection. However, detection speed and selectivity of MOS-based sensors currently face great challenges. Herein, we design palladium single atoms (SAs) doped tin oxide (SnO2/Pdatom) for H2 detection. Actual sensing tests show an ultrafast response speed toward H2 (3s to 10 ppm H2), with detection limit of 50 ppb and superior selectivity. Using in-situ THz time-domain spectroscopy and density functional theory calculations, it proves that an extra energy band near Fermi level appeared in SnO2/Pdatom, and Pd SAs doped on SnO2 enhance signally concentration of free carrier in SnO2/Pdatom. Partial density of states reveals that coupling hybridization between Pd 4d orbital and O 2p orbital promotes electron injection from Pd 4d orbital into O π2p orbital, improving production of more O- ions on sensing surfaces. Consequentially, the sensing dynamics involving O- ions spillover at SnO2-Pdatom interface is discussed.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s43246-025-00865-5
- https://www.nature.com/articles/s43246-025-00865-5.pdf
- OA Status
- gold
- Cited By
- 2
- References
- 59
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4412020396
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4412020396Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s43246-025-00865-5Digital Object Identifier
- Title
-
Hydrogen sensing with high-performance via O- ion spillover at Pd single atoms stabilized SnO2 interfaceWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2025Year of publication
- Publication date
-
2025-07-04Full publication date if available
- Authors
-
Yinyin Qian, Guorui Zhao, Changming Zhang, Shengjie Yin, Junwei Chen, Yuanyuan Luo, Zhengfeng Huang, Bo Liu, Guotao DuanList of authors in order
- Landing page
-
https://doi.org/10.1038/s43246-025-00865-5Publisher landing page
- PDF URL
-
https://www.nature.com/articles/s43246-025-00865-5.pdfDirect link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
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https://www.nature.com/articles/s43246-025-00865-5.pdfDirect OA link when available
- Concepts
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Ion, Interface (matter), Spillover effect, Hydrogen, Materials science, Optoelectronics, Chemistry, Composite material, Economics, Organic chemistry, Microeconomics, Capillary number, Capillary actionTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
2Total citation count in OpenAlex
- Citations by year (recent)
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2025: 2Per-year citation counts (last 5 years)
- References (count)
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59Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W3101586829, https://openalex.org/W4389233003, https://openalex.org/W3162628218, https://openalex.org/W4403706867, https://openalex.org/W3096338351, https://openalex.org/W4404238272, https://openalex.org/W2346162438, https://openalex.org/W4403260132, https://openalex.org/W4394572716, https://openalex.org/W4400964746, https://openalex.org/W4380577421, https://openalex.org/W2973754009, https://openalex.org/W2743876723, https://openalex.org/W2793852832, https://openalex.org/W2193077821, https://openalex.org/W4383878834, https://openalex.org/W3174678097, https://openalex.org/W2322474936, https://openalex.org/W2802791016, https://openalex.org/W3210306354, https://openalex.org/W4295905321, https://openalex.org/W4320727642, https://openalex.org/W4297977999, https://openalex.org/W4399107374, https://openalex.org/W4384156087, https://openalex.org/W4214514888, https://openalex.org/W3166527874, https://openalex.org/W2893880082, https://openalex.org/W3152794426, https://openalex.org/W3009261750, https://openalex.org/W4310948665, https://openalex.org/W4372279822, https://openalex.org/W3167441965, https://openalex.org/W2964813318, https://openalex.org/W4391025977, https://openalex.org/W1984315444, https://openalex.org/W2075961933, https://openalex.org/W2052810663, https://openalex.org/W3082485318, https://openalex.org/W4307971163, https://openalex.org/W4392844667, https://openalex.org/W2542089834, https://openalex.org/W2070070389, https://openalex.org/W2773596263, https://openalex.org/W4211056445, https://openalex.org/W2064828060, https://openalex.org/W1957310144, https://openalex.org/W4406894028, https://openalex.org/W2619025018, https://openalex.org/W4385850927, https://openalex.org/W4295296119, https://openalex.org/W3016880118, https://openalex.org/W2025162195, https://openalex.org/W2106223635, https://openalex.org/W2007395042, https://openalex.org/W2083222334, https://openalex.org/W1981368803, https://openalex.org/W1979544533, https://openalex.org/W2036113194 |
| referenced_works_count | 59 |
| abstract_inverted_index.O | 134, 145 |
| abstract_inverted_index.a | 28 |
| abstract_inverted_index.10 | 72 |
| abstract_inverted_index.2p | 135 |
| abstract_inverted_index.4d | 131, 142 |
| abstract_inverted_index.50 | 79 |
| abstract_inverted_index.H2 | 32, 58, 69 |
| abstract_inverted_index.O- | 152, 162 |
| abstract_inverted_index.Pd | 108, 130, 141 |
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| abstract_inverted_index.in | 105, 119 |
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| abstract_inverted_index.we | 47 |
| abstract_inverted_index.(3s | 70 |
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| abstract_inverted_index.THz | 86 |
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| abstract_inverted_index.H2), | 74 |
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| abstract_inverted_index.oxide | 14, 55 |
| abstract_inverted_index.speed | 36, 67 |
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| abstract_inverted_index.Actual | 60 |
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| abstract_inverted_index.proves | 95 |
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| abstract_inverted_index.detection. | 33, 59 |
| abstract_inverted_index.discussed. | 169 |
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| abstract_inverted_index.imperative | 8 |
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| abstract_inverted_index.SnO2-Pdatom | 166 |
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| abstract_inverted_index.semiconductor | 15 |
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| sustainable_development_goals[0].display_name | Affordable and clean energy |
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