Identifying critical features of iron phosphate particle for lithium preference Article Swipe
Gangbin Yan
,
Jialiang Wei
,
Emory Apodaca
,
Suin Choi
,
Peter J. Eng
,
Joanne E. Stubbs
,
Yu Han
,
Siqi Zou
,
Mrinal K. Bera
,
Ronghui Wu
,
Evguenia Karapetrova
,
Hua Zhou
,
Wei Chen
,
Chong Liu
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-024-49191-3
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-024-49191-3
One-dimensional (1D) olivine iron phosphate (FePO 4 ) is widely proposed for electrochemical lithium (Li) extraction from dilute water sources, however, significant variations in Li selectivity were observed for particles with different physical attributes. Understanding how particle features influence Li and sodium (Na) co-intercalation is crucial for system design and enhancing Li selectivity. Here, we investigate a series of FePO 4 particles with various features and revealed the importance of harnessing kinetic and chemo-mechanical barrier difference between lithiation and sodiation to promote selectivity. The thermodynamic preference of FePO 4 provides baseline of selectivity while the particle features are critical to induce different kinetic pathways and barriers, resulting in different Li to Na selectivity from 6.2 × 10 2 to 2.3 × 10 4 . Importantly, we categorize the FePO 4 particles into two groups based on their distinctly paired phase evolutions upon lithiation and sodiation, and generate quantitative correlation maps among Li preference, morphological features, and electrochemical properties. By selecting FePO 4 particles with specific features, we demonstrate fast (636 mA/g) Li extraction from a high Li source (1: 100 Li to Na) with (96.6 ± 0.2)% purity, and high selectivity (2.3 × 10 4 ) from a low Li source (1: 1000 Li to Na) with (95.8 ± 0.3)% purity in a single step.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41467-024-49191-3
- https://www.nature.com/articles/s41467-024-49191-3.pdf
- OA Status
- gold
- Cited By
- 15
- References
- 44
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4399438864
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Raw OpenAlex JSON
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https://openalex.org/W4399438864Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41467-024-49191-3Digital Object Identifier
- Title
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Identifying critical features of iron phosphate particle for lithium preferenceWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-06-07Full publication date if available
- Authors
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Gangbin Yan, Jialiang Wei, Emory Apodaca, Suin Choi, Peter J. Eng, Joanne E. Stubbs, Yu Han, Siqi Zou, Mrinal K. Bera, Ronghui Wu, Evguenia Karapetrova, Hua Zhou, Wei Chen, Chong LiuList of authors in order
- Landing page
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https://doi.org/10.1038/s41467-024-49191-3Publisher landing page
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https://www.nature.com/articles/s41467-024-49191-3.pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.nature.com/articles/s41467-024-49191-3.pdfDirect OA link when available
- Concepts
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Lithium iron phosphate, Lithium (medication), Phosphate, Particle (ecology), Preference, Iron phosphate, Chemistry, Computer science, Computational biology, Biology, Biochemistry, Mathematics, Ecology, Statistics, Electrode, Physical chemistry, Endocrinology, ElectrochemistryTop concepts (fields/topics) attached by OpenAlex
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15Total citation count in OpenAlex
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2025: 12, 2024: 3Per-year citation counts (last 5 years)
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44Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.olivine | 3 |
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| abstract_inverted_index.purity, | 188 |
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| abstract_inverted_index.particles | 30, 62, 131, 163 |
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| abstract_inverted_index.selecting | 160 |
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| abstract_inverted_index.importance | 69 |
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| abstract_inverted_index.preference | 86 |
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| abstract_inverted_index.chemo-mechanical | 74 |
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| cited_by_percentile_year.min | 96 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 14 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/6 |
| sustainable_development_goals[0].score | 0.8600000143051147 |
| sustainable_development_goals[0].display_name | Clean water and sanitation |
| citation_normalized_percentile.value | 0.95073562 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |