In Situ Tuning of Catalytic Activity by Thermoelectric Effect for Ethylene Oxidation Article Swipe
Abdenour Achour
,
Jian Liu
,
Ping Peng
,
Christopher Shaw
,
Z. Huang
·
YOU?
·
· 2018
· Open Access
·
· DOI: https://doi.org/10.1021/acscatal.8b02409
YOU?
·
· 2018
· Open Access
·
· DOI: https://doi.org/10.1021/acscatal.8b02409
Thermoelectric material BiCuSeO used as a support and promoter for catalytic ethylene oxidation is reported here. The catalytic activity on the continuous and non-continuous catalyst Pt supported on BiCuSeO was observed to be promoted in-situ by a thermoelectric Seebeck voltage generated by the temperature gradient across the material. It is also shown this thermoelectric promotion of catalysis enabled the thermoelectric material BiCuSeO itself to be highly catalytic active for ethylene oxidation. A good linear relationship between the logarithm of the reaction rate and the thermoelectric Seebeck voltage was observed. This thermoelectric promotion of catalysis is attributed to the change of work function of the catalyst surface, accompanied by a charge transfer from the bulk to the surface due to the thermoelectric effect.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acscatal.8b02409
- OA Status
- green
- Cited By
- 29
- References
- 39
- Related Works
- 10
- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W2891525555Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1021/acscatal.8b02409Digital Object Identifier
- Title
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In Situ Tuning of Catalytic Activity by Thermoelectric Effect for Ethylene OxidationWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2018Year of publication
- Publication date
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2018-09-20Full publication date if available
- Authors
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Abdenour Achour, Jian Liu, Ping Peng, Christopher Shaw, Z. HuangList of authors in order
- Landing page
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https://doi.org/10.1021/acscatal.8b02409Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
- OA URL
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https://dspace.lib.cranfield.ac.uk/handle/1826/13491Direct OA link when available
- Concepts
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Thermoelectric effect, Catalysis, Materials science, Seebeck coefficient, Ethylene, Thermoelectric materials, Chemical engineering, Work function, Metal, Chemistry, Metallurgy, Organic chemistry, Thermodynamics, Physics, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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29Total citation count in OpenAlex
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2025: 4, 2024: 6, 2023: 5, 2022: 4, 2021: 5Per-year citation counts (last 5 years)
- References (count)
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39Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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