Incipient Ionic Conductors: Ion‐Constrained Lattices Achieving Superionic‐Like Thermal Conductivity Through Extreme Anharmonicity Article Swipe
Yongheng Li
,
Qiuchun Lu
,
Bin Wei
,
Cong Lu
,
Xingang Jiang
,
Taishun Manjo
,
Daisuke Ishikawa
,
Caofeng Pan
,
Alfred Q. R. Baron
,
Jiawang Hong
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202513381
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/adma.202513381
Phonon liquid‐like thermal conduction in the solid state enables superionic conductors to serve as efficient thermoelectric device candidates. While liquid‐like motion of ions effectively suppresses thermal conductivity ( κ ), their high mobility concurrently triggers material degradation due to undesirable ion migration and consequent metal deposition, making it a challenge to balance low κ and high stability. Here, phonon liquid‐like thermal transport is reported alongside restricted long‐range ion migration in CsCu 2 I 3 with incipient ionic conduction, using synchrotron X‐ray diffraction, inelastic X‐ray scattering, and machine‐learning potential‐based simulations. The Cu ions are revealed to exhibit confined migration between CuI 4 tetrahedra at high temperatures, displaying extreme anharmonicity of dominated phonons beyond conventional rattling and comparable to that in superionic conductors. Consequently, a glass‐like κ (≈0.3 W m −1 K −1 at 300 K) following the relationship of κ ≈ T 0.17 , is achieved along the x ‐direction, where Cu ion migration is three orders of magnitude lower than in superionic conductors. These results highlight the advantage of incipient ionic conductors in simultaneously maintaining both low κ and high stability, elucidating the thermal transport mechanism via ion migration constraints, and paving an effective pathway toward ultralow thermal conductivity in ionic conductors.
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- OA Status
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- 58
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Incipient Ionic Conductors: Ion‐Constrained Lattices Achieving Superionic‐Like Thermal Conductivity Through Extreme AnharmonicityWork title
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articleOpenAlex work type
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enPrimary language
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2025Year of publication
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2025-09-15Full publication date if available
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Yongheng Li, Qiuchun Lu, Bin Wei, Cong Lu, Xingang Jiang, Taishun Manjo, Daisuke Ishikawa, Caofeng Pan, Alfred Q. R. Baron, Jiawang HongList of authors in order
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