Induced Manipulation of Atomically Dispersed Cobalt through S Vacancy for Photocatalytic Water Splitting: Asymmetric Coordination and Dynamic Evolution Article Swipe
Meixue Chen
,
Minhao Li
,
Shuqu Zhang
,
Xia Liu
,
Lixia Yang
,
Ren‐Jie Song
,
Jian‐Ping Zou
,
Shenglian Luo
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/advs.202405137
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/advs.202405137
It is still a challenge to construct single‐atom level reduction and oxidation sites in single‐component photocatalyst by manipulating coordination configuration for photocatalytic water splitting. Herein, the atomically dispersed asymmetric configuration of six‐coordinated Co‐S 2 O 4 (two exposed S atoms, two OH groups, and two Co─O─Zn bonds) suspending on ZnIn 2 S 4 nanosheets verified by combining experimental analysis with theoretical calculation, is applied into photocatalytic water splitting. The Co‐S 2 O 4 site immobilized by Vs acts as oxidation sites to guide electrons transferring to neighboring independent S atom, achieving efficient separation of reduction and oxidation sites. It is worth mentioning that stabilized Co‐S 2 O 4 configuration show dynamic structure evolution to highly active Co‐S 1 O 4 configuration (one exposed S atom, one OH group, and three Co─O─Zn bonds) in reaction, which lowers energy barrier of transition state for H 2 O activization. Ultimately, the optimized photocatalyst exhibits excellent photocatalytic activity for water splitting (H 2 : 80.13 µmol g −1 h −1 , O 2 : 37.81 µmol g −1 h −1 ) and outstanding stability than that of multicomponent photocatalysts due to dynamic and reversible evolution between stable Co‐S 2 O 4 configuration and active Co‐S 1 O 4 configuration. This work demonstrates new cognitions on immobilized strategy through vacancy inducing, manipulating coordination configuration, and dynamic evolution mechanism of single‐atom level catalytic site in photocatalytic water splitting.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/advs.202405137
- OA Status
- gold
- Cited By
- 10
- References
- 38
- Related Works
- 10
- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4401554572Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/advs.202405137Digital Object Identifier
- Title
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Induced Manipulation of Atomically Dispersed Cobalt through S Vacancy for Photocatalytic Water Splitting: Asymmetric Coordination and Dynamic EvolutionWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-08-13Full publication date if available
- Authors
-
Meixue Chen, Minhao Li, Shuqu Zhang, Xia Liu, Lixia Yang, Ren‐Jie Song, Jian‐Ping Zou, Shenglian LuoList of authors in order
- Landing page
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https://doi.org/10.1002/advs.202405137Publisher landing page
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1002/advs.202405137Direct OA link when available
- Concepts
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Photocatalysis, Cobalt, Vacancy defect, Water splitting, Materials science, Chemical engineering, Chemical physics, Nanotechnology, Crystallography, Chemistry, Metallurgy, Catalysis, Engineering, BiochemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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10Total citation count in OpenAlex
- Citations by year (recent)
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2025: 9, 2024: 1Per-year citation counts (last 5 years)
- References (count)
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38Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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