Influence of Cellulose Nanofibers on the Behavior of Pickering Emulsions. Part 1. Microscopy and Startup Flow Test Article Swipe
Shuming Cui
,
Saud Hashmi
,
Wenqiang Li
,
Stephan Handschuh‐Wang
,
Cheng-Tian Zhu
,
Shichang Wang
,
Pianpian Yang
,
Yanfei Huang
,
Guangming Zhu
,
Florian J. Stadler
·
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/ma15238285
YOU?
·
· 2022
· Open Access
·
· DOI: https://doi.org/10.3390/ma15238285
The dispersibility of flexible polymer chains present at the emulsion’s interface between the dispersed and continuous phase has obvious effects on rheology and dielectric properties of the whole emulsion. Cellulose nanofiber (CNF)-based Pickering emulsions are good systems to research these properties with respect to their microscopic phase structure, dielectric, and rheological properties by using CNF as a water-dispersible Pickering emulsifier, liquid paraffin as an oil phase, and didodecyldimethylammonium bromide (DDAB) as a cationic auxiliary surfactant. The CNF and DDAB contents were systematically varied while the water-to-paraffin oil ratio was kept constant to discern the influence of the Pickering emulsifiers. Polarized optical microscopic images reveal that the droplets tend to shrink at higher CNF content but grow bigger when increasing the DDAB content, which is proved by fluorescence analysis of the CNF dispersibility with varying DDAB content. The dielectric damping exhibits a minimum, whose value decreases with increasing DDAB and CNF content. Increasing the DDAB content promotes the solubilization of CNF in the aqueous phase, which will increase the overall viscosity and yield points. Similarly, a higher CNF content leads to a higher viscosity and yield point, but at high DDAB contents, the viscosity function exhibits an S-shape at intermediate CNF contents. To evaluate the results further, they were compared with CNF dispersions (without oil phase), which showed a surfactant effect slightly on maximum stress but strongly on yield stress τy, indicating that DDAB can promote the formation of a CNF network rather than the viscosity of the whole system. This paper provides information on how a systematical variation of the composition influences morphology and physico-chemical interactions as detected by broadband dielectric spectroscopy and rheological behavior.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/ma15238285
- https://www.mdpi.com/1996-1944/15/23/8285/pdf?version=1670406368
- OA Status
- gold
- Cited By
- 3
- References
- 65
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4309588550
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Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4309588550Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/ma15238285Digital Object Identifier
- Title
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Influence of Cellulose Nanofibers on the Behavior of Pickering Emulsions. Part 1. Microscopy and Startup Flow TestWork title
- Type
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articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2022Year of publication
- Publication date
-
2022-11-22Full publication date if available
- Authors
-
Shuming Cui, Saud Hashmi, Wenqiang Li, Stephan Handschuh‐Wang, Cheng-Tian Zhu, Shichang Wang, Pianpian Yang, Yanfei Huang, Guangming Zhu, Florian J. StadlerList of authors in order
- Landing page
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https://doi.org/10.3390/ma15238285Publisher landing page
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https://www.mdpi.com/1996-1944/15/23/8285/pdf?version=1670406368Direct link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.mdpi.com/1996-1944/15/23/8285/pdf?version=1670406368Direct OA link when available
- Concepts
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Rheology, Pickering emulsion, Materials science, Chemical engineering, Pulmonary surfactant, Viscosity, Emulsion, Yield (engineering), Phase (matter), Cationic polymerization, Cellulose, Polymer chemistry, Composite material, Organic chemistry, Chemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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3Total citation count in OpenAlex
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2025: 1, 2024: 1, 2023: 1Per-year citation counts (last 5 years)
- References (count)
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65Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.emulsifiers. | 98 |
| abstract_inverted_index.emulsion’s | 9 |
| abstract_inverted_index.fluorescence | 126 |
| abstract_inverted_index.interactions | 265 |
| abstract_inverted_index.intermediate | 198 |
| abstract_inverted_index.spectroscopy | 271 |
| abstract_inverted_index.systematical | 256 |
| abstract_inverted_index.dispersibility | 1, 131 |
| abstract_inverted_index.solubilization | 157 |
| abstract_inverted_index.systematically | 81 |
| abstract_inverted_index.physico-chemical | 264 |
| abstract_inverted_index.water-dispersible | 57 |
| abstract_inverted_index.water-to-paraffin | 85 |
| abstract_inverted_index.didodecyldimethylammonium | 67 |
| cited_by_percentile_year.max | 95 |
| cited_by_percentile_year.min | 89 |
| corresponding_author_ids | https://openalex.org/A5102876130, https://openalex.org/A5073987958, https://openalex.org/A5030266953 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 10 |
| corresponding_institution_ids | https://openalex.org/I180726961 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/6 |
| sustainable_development_goals[0].score | 0.8199999928474426 |
| sustainable_development_goals[0].display_name | Clean water and sanitation |
| citation_normalized_percentile.value | 0.52440377 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |