Influence of the Acid Reactivity of Carbenium Ions in Zeolites on the Methanol‐to‐Olefins Process Article Swipe
Luca Maggiulli
,
Vitaly L. Sushkevich
,
Annika E. Enss
,
Felix Studt
,
Jeroen A. van Bokhoven
,
Davide Ferri
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/anie.202514759
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/anie.202514759
Carbocations are typical intermediates in acid catalyzed reactions in organic chemistry synthesis. Confinement within the framework of zeotype materials distinguishes the function of carbenium ions as catalytic centers in various chemical processes. A selective and reversible deprotonation event of benzenium ions built in H‐ZSM‐5 during methanol conversion was observed by experiment and theory as a result of CD 3 CN dosage, denoting their higher acid reactivity compared to the cyclopentenyl cations, which undergo deprotonation only in presence of pyridine. This study uncovers the inverse relationship between the acid reactivity of carbenium ions of different nature and their stability in the surface‐bound state.
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Influence of the Acid Reactivity of Carbenium Ions in Zeolites on the Methanol‐to‐Olefins ProcessWork title
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Luca Maggiulli, Vitaly L. Sushkevich, Annika E. Enss, Felix Studt, Jeroen A. van Bokhoven, Davide FerriList of authors in order
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| abstract_inverted_index.3 | 59 |
| abstract_inverted_index.A | 33 |
| abstract_inverted_index.a | 55 |
| abstract_inverted_index.CD | 58 |
| abstract_inverted_index.CN | 60 |
| abstract_inverted_index.as | 26, 54 |
| abstract_inverted_index.by | 50 |
| abstract_inverted_index.in | 5, 9, 29, 43, 76, 99 |
| abstract_inverted_index.of | 17, 23, 39, 57, 78, 90, 93 |
| abstract_inverted_index.to | 68 |
| abstract_inverted_index.and | 35, 52, 96 |
| abstract_inverted_index.are | 2 |
| abstract_inverted_index.the | 15, 21, 69, 83, 87, 100 |
| abstract_inverted_index.was | 48 |
| abstract_inverted_index.This | 80 |
| abstract_inverted_index.acid | 6, 65, 88 |
| abstract_inverted_index.ions | 25, 41, 92 |
| abstract_inverted_index.only | 75 |
| abstract_inverted_index.built | 42 |
| abstract_inverted_index.event | 38 |
| abstract_inverted_index.study | 81 |
| abstract_inverted_index.their | 63, 97 |
| abstract_inverted_index.which | 72 |
| abstract_inverted_index.during | 45 |
| abstract_inverted_index.higher | 64 |
| abstract_inverted_index.nature | 95 |
| abstract_inverted_index.result | 56 |
| abstract_inverted_index.state. | 102 |
| abstract_inverted_index.theory | 53 |
| abstract_inverted_index.within | 14 |
| abstract_inverted_index.between | 86 |
| abstract_inverted_index.centers | 28 |
| abstract_inverted_index.dosage, | 61 |
| abstract_inverted_index.inverse | 84 |
| abstract_inverted_index.organic | 10 |
| abstract_inverted_index.typical | 3 |
| abstract_inverted_index.undergo | 73 |
| abstract_inverted_index.various | 30 |
| abstract_inverted_index.zeotype | 18 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.cations, | 71 |
| abstract_inverted_index.chemical | 31 |
| abstract_inverted_index.compared | 67 |
| abstract_inverted_index.denoting | 62 |
| abstract_inverted_index.function | 22 |
| abstract_inverted_index.methanol | 46 |
| abstract_inverted_index.observed | 49 |
| abstract_inverted_index.presence | 77 |
| abstract_inverted_index.uncovers | 82 |
| abstract_inverted_index.benzenium | 40 |
| abstract_inverted_index.carbenium | 24, 91 |
| abstract_inverted_index.catalytic | 27 |
| abstract_inverted_index.catalyzed | 7 |
| abstract_inverted_index.chemistry | 11 |
| abstract_inverted_index.different | 94 |
| abstract_inverted_index.framework | 16 |
| abstract_inverted_index.materials | 19 |
| abstract_inverted_index.pyridine. | 79 |
| abstract_inverted_index.reactions | 8 |
| abstract_inverted_index.selective | 34 |
| abstract_inverted_index.stability | 98 |
| abstract_inverted_index.conversion | 47 |
| abstract_inverted_index.experiment | 51 |
| abstract_inverted_index.processes. | 32 |
| abstract_inverted_index.reactivity | 66, 89 |
| abstract_inverted_index.reversible | 36 |
| abstract_inverted_index.synthesis. | 12 |
| abstract_inverted_index.Confinement | 13 |
| abstract_inverted_index.H‐ZSM‐5 | 44 |
| abstract_inverted_index.Carbocations | 1 |
| abstract_inverted_index.relationship | 85 |
| abstract_inverted_index.cyclopentenyl | 70 |
| abstract_inverted_index.deprotonation | 37, 74 |
| abstract_inverted_index.distinguishes | 20 |
| abstract_inverted_index.intermediates | 4 |
| abstract_inverted_index.surface‐bound | 101 |
| cited_by_percentile_year | |
| corresponding_author_ids | https://openalex.org/A5054120563, https://openalex.org/A5041651435 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 6 |
| corresponding_institution_ids | https://openalex.org/I2802229908, https://openalex.org/I35440088, https://openalex.org/I4210092485 |
| citation_normalized_percentile.value | 0.46248477 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |