Infrared Imaging using thermally stable HgTe/CdS nanocrystals Article Swipe
Huichen Zhang
,
Yoann Prado
,
Rodolphe Alchaar
,
Henri Lehouelleur
,
Mariarosa Cavallo
,
Tung Huu Dang
,
Adrien Khalili
,
Erwan Bossavit
,
Corentin Dabard
,
Nicolas Ledos
,
Mathieu G. Silly
,
Ali Madouri
,
Danièle Fournier
,
James K. Utterback
,
Debora Pierucci
,
Victor Parahyba
,
Pierre Potet
,
David Darson
,
Sandrine Ithurria
,
B. Szafran
,
Benjamin T. Diroll
,
Juan I. Climente
,
Emmanuel Lhuillier
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2402.13745
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.2402.13745
Transferring the nanocrystals (NCs) from the laboratory environment toward practical applications has raised new challenges. In the case of NCs for display and lightning, the focus was on reduced Auger recombination and maintaining luminescence at high temperatures. When it comes to infrared sensing, narrow band gap materials are required and HgTe appears as the most spectrally tunable platform. Its low-temperature synthesis reduces the growth energy cost yet also favors sintering. As a result, once coupled to a read-out circuit, the Joule effect aggregates the particles leading to a poorly defined optical edge and dramatically large dark current. Here, we demonstrate that CdS shells bring the expected thermal stability (no redshift upon annealing, reduced tendency to form amalgams and preservation of photoconduction after an atomic layer deposition process). The peculiar electronic structure of these confined particles is unveiled using k.p self-consistent simulations showing a significant exciton biding energy at around 200 meV. After shelling, the material displays a p-type behavior that favors the generation of photoconductive gain. The latter is then used to increase the external quantum
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Metadata
- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/2402.13745
- https://arxiv.org/pdf/2402.13745
- OA Status
- green
- Cited By
- 2
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4392090009
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4392090009Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.2402.13745Digital Object Identifier
- Title
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Infrared Imaging using thermally stable HgTe/CdS nanocrystalsWork title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-02-21Full publication date if available
- Authors
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Huichen Zhang, Yoann Prado, Rodolphe Alchaar, Henri Lehouelleur, Mariarosa Cavallo, Tung Huu Dang, Adrien Khalili, Erwan Bossavit, Corentin Dabard, Nicolas Ledos, Mathieu G. Silly, Ali Madouri, Danièle Fournier, James K. Utterback, Debora Pierucci, Victor Parahyba, Pierre Potet, David Darson, Sandrine Ithurria, B. Szafran, Benjamin T. Diroll, Juan I. Climente, Emmanuel LhuillierList of authors in order
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https://arxiv.org/abs/2402.13745Publisher landing page
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https://arxiv.org/pdf/2402.13745Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
greenOpen access status per OpenAlex
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https://arxiv.org/pdf/2402.13745Direct OA link when available
- Concepts
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Nanocrystal, Infrared, Optoelectronics, Materials science, Nanotechnology, Optics, PhysicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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2Total citation count in OpenAlex
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2025: 1, 2024: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.to | 40, 75, 86, 114, 171 |
| abstract_inverted_index.we | 98 |
| abstract_inverted_index.(no | 108 |
| abstract_inverted_index.200 | 149 |
| abstract_inverted_index.CdS | 101 |
| abstract_inverted_index.Its | 58 |
| abstract_inverted_index.NCs | 19 |
| abstract_inverted_index.The | 127, 166 |
| abstract_inverted_index.and | 22, 31, 49, 92, 117 |
| abstract_inverted_index.are | 47 |
| abstract_inverted_index.for | 20 |
| abstract_inverted_index.gap | 45 |
| abstract_inverted_index.has | 11 |
| abstract_inverted_index.k.p | 138 |
| abstract_inverted_index.new | 13 |
| abstract_inverted_index.the | 1, 5, 16, 24, 53, 62, 79, 83, 104, 153, 161, 173 |
| abstract_inverted_index.was | 26 |
| abstract_inverted_index.yet | 66 |
| abstract_inverted_index.HgTe | 50 |
| abstract_inverted_index.When | 37 |
| abstract_inverted_index.also | 67 |
| abstract_inverted_index.band | 44 |
| abstract_inverted_index.case | 17 |
| abstract_inverted_index.cost | 65 |
| abstract_inverted_index.dark | 95 |
| abstract_inverted_index.edge | 91 |
| abstract_inverted_index.form | 115 |
| abstract_inverted_index.from | 4 |
| abstract_inverted_index.high | 35 |
| abstract_inverted_index.meV. | 150 |
| abstract_inverted_index.most | 54 |
| abstract_inverted_index.once | 73 |
| abstract_inverted_index.that | 100, 159 |
| abstract_inverted_index.then | 169 |
| abstract_inverted_index.upon | 110 |
| abstract_inverted_index.used | 170 |
| abstract_inverted_index.(NCs) | 3 |
| abstract_inverted_index.After | 151 |
| abstract_inverted_index.Auger | 29 |
| abstract_inverted_index.Here, | 97 |
| abstract_inverted_index.Joule | 80 |
| abstract_inverted_index.after | 121 |
| abstract_inverted_index.bring | 103 |
| abstract_inverted_index.comes | 39 |
| abstract_inverted_index.focus | 25 |
| abstract_inverted_index.gain. | 165 |
| abstract_inverted_index.large | 94 |
| abstract_inverted_index.layer | 124 |
| abstract_inverted_index.these | 132 |
| abstract_inverted_index.using | 137 |
| abstract_inverted_index.around | 148 |
| abstract_inverted_index.atomic | 123 |
| abstract_inverted_index.biding | 145 |
| abstract_inverted_index.effect | 81 |
| abstract_inverted_index.energy | 64, 146 |
| abstract_inverted_index.favors | 68, 160 |
| abstract_inverted_index.growth | 63 |
| abstract_inverted_index.latter | 167 |
| abstract_inverted_index.narrow | 43 |
| abstract_inverted_index.p-type | 157 |
| abstract_inverted_index.poorly | 88 |
| abstract_inverted_index.raised | 12 |
| abstract_inverted_index.shells | 102 |
| abstract_inverted_index.toward | 8 |
| abstract_inverted_index.appears | 51 |
| abstract_inverted_index.coupled | 74 |
| abstract_inverted_index.defined | 89 |
| abstract_inverted_index.display | 21 |
| abstract_inverted_index.exciton | 144 |
| abstract_inverted_index.leading | 85 |
| abstract_inverted_index.optical | 90 |
| abstract_inverted_index.quantum | 175 |
| abstract_inverted_index.reduced | 28, 112 |
| abstract_inverted_index.reduces | 61 |
| abstract_inverted_index.result, | 72 |
| abstract_inverted_index.showing | 141 |
| abstract_inverted_index.thermal | 106 |
| abstract_inverted_index.tunable | 56 |
| abstract_inverted_index.amalgams | 116 |
| abstract_inverted_index.behavior | 158 |
| abstract_inverted_index.circuit, | 78 |
| abstract_inverted_index.confined | 133 |
| abstract_inverted_index.current. | 96 |
| abstract_inverted_index.displays | 155 |
| abstract_inverted_index.expected | 105 |
| abstract_inverted_index.external | 174 |
| abstract_inverted_index.increase | 172 |
| abstract_inverted_index.infrared | 41 |
| abstract_inverted_index.material | 154 |
| abstract_inverted_index.peculiar | 128 |
| abstract_inverted_index.read-out | 77 |
| abstract_inverted_index.redshift | 109 |
| abstract_inverted_index.required | 48 |
| abstract_inverted_index.sensing, | 42 |
| abstract_inverted_index.tendency | 113 |
| abstract_inverted_index.unveiled | 136 |
| abstract_inverted_index.materials | 46 |
| abstract_inverted_index.particles | 84, 134 |
| abstract_inverted_index.platform. | 57 |
| abstract_inverted_index.practical | 9 |
| abstract_inverted_index.process). | 126 |
| abstract_inverted_index.shelling, | 152 |
| abstract_inverted_index.stability | 107 |
| abstract_inverted_index.structure | 130 |
| abstract_inverted_index.synthesis | 60 |
| abstract_inverted_index.aggregates | 82 |
| abstract_inverted_index.annealing, | 111 |
| abstract_inverted_index.deposition | 125 |
| abstract_inverted_index.electronic | 129 |
| abstract_inverted_index.generation | 162 |
| abstract_inverted_index.laboratory | 6 |
| abstract_inverted_index.lightning, | 23 |
| abstract_inverted_index.sintering. | 69 |
| abstract_inverted_index.spectrally | 55 |
| abstract_inverted_index.challenges. | 14 |
| abstract_inverted_index.demonstrate | 99 |
| abstract_inverted_index.environment | 7 |
| abstract_inverted_index.maintaining | 32 |
| abstract_inverted_index.significant | 143 |
| abstract_inverted_index.simulations | 140 |
| abstract_inverted_index.Transferring | 0 |
| abstract_inverted_index.applications | 10 |
| abstract_inverted_index.dramatically | 93 |
| abstract_inverted_index.luminescence | 33 |
| abstract_inverted_index.nanocrystals | 2 |
| abstract_inverted_index.preservation | 118 |
| abstract_inverted_index.recombination | 30 |
| abstract_inverted_index.temperatures. | 36 |
| abstract_inverted_index.low-temperature | 59 |
| abstract_inverted_index.photoconduction | 120 |
| abstract_inverted_index.photoconductive | 164 |
| abstract_inverted_index.self-consistent | 139 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 23 |
| citation_normalized_percentile |