Insight Into Pre‐Intercalation of Layered Vanadium Oxide Cathodes: From Precise Control of the Interspace to Related Electrochemical Performance and Beyond Article Swipe
Zhangxiang Hao
,
Jian Wang
,
Junrun Feng
,
Yameng Fan
,
Jian Peng
,
Jiazhao Wang
,
Shi Xue Dou
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/cey2.681
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/cey2.681
Pre‐intercalation is the mainstream approach to inhibit the unpredicted structural degradation and the sluggish kinetics of Zn‐ions migrating in vanadium oxide cathode of aqueous zinc‐ion batteries (AZIBs), which has been extensively explored over the past 5 years. The functional principles behind the improvement are widely discussed but have been limited to the enlargement of interspace between VO layers. As the different types of ions could change the properties of vanadium oxides in various ways, the review starts with a comprehensive overview of pre‐intercalated vanadium oxide cathode with different types of molecules and ions, such as metal ions, water molecules, and non‐metallic cations, along with their functional principles and resulting performance. Furthermore, the pre‐intercalated vanadium cathodes reported so far are summarized, comparing their interlayer space, capacity, cycling rate, and capacity retention after long cycling. A discussion of the relationship between the interspace and the performance is provided. The widest interspaces could result in the decay of the cycling stability. Based on the data, the optimal interspace is likely to be around 12 Å, indicating that precise control of the interspace is a useful method. However, more consideration is required regarding the other impacts of pre‐intercalated ions on vanadium oxide. It is hoped that this review can inspire further understanding of pre‐intercalated vanadium oxide cathodes, paving a new pathway to the development of advanced vanadium oxide cathodes with better cycling stability and larger energy density.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/cey2.681
- OA Status
- gold
- Cited By
- 14
- References
- 104
- Related Works
- 10
- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4408332963Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/cey2.681Digital Object Identifier
- Title
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Insight Into Pre‐Intercalation of Layered Vanadium Oxide Cathodes: From Precise Control of the Interspace to Related Electrochemical Performance and BeyondWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-02-27Full publication date if available
- Authors
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Zhangxiang Hao, Jian Wang, Junrun Feng, Yameng Fan, Jian Peng, Jiazhao Wang, Shi Xue DouList of authors in order
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https://doi.org/10.1002/cey2.681Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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goldOpen access status per OpenAlex
- OA URL
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https://doi.org/10.1002/cey2.681Direct OA link when available
- Concepts
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Intercalation (chemistry), Vanadium oxide, Electrochemistry, Cathode, Vanadium, Oxide, Materials science, Nanotechnology, Inorganic chemistry, Chemistry, Metallurgy, Electrode, Physical chemistryTop concepts (fields/topics) attached by OpenAlex
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14Total citation count in OpenAlex
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2025: 14Per-year citation counts (last 5 years)
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104Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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