Integrated a Fused Silica Capillary Cell and In Situ Raman Spectroscopy for Determining the Solubility of CO2 in n-Decane and n-Decane + n-Hexane System Article Swipe
Junliang Wang
,
Zhenzhen Zhang
,
Quanyuan Wang
,
Tianhong Lou
,
Zhiyan Pan
,
Mian Hu
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.3390/pr11041137
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.3390/pr11041137
Understanding the solubility of CO2 is critical for implementing CO2-enhanced oil recovery (CO2-EOR). In this work, the solubility of CO2 in n-decane in a temperature range between 303.15 K and 353.15 K and pressures up to 15 MPa was measured using a fused silica capillary cell with in situ Raman spectroscopy. A semi-empirical CO2 solubility prediction model was obtained according to the experimental results. In order to improve the solubility of CO2 in n-decane, the solubility of CO2 in n-decane and co-solvent n-hexane (3% wt) mixture was also comparatively investigated. The results indicated that the solubility of CO2 in n-decane was 1.6355~64.0084 mol/kg. The data from the prediction model were in good agreement with the experimental data, and the mean relative deviation was 3.65%, indicating that the prediction model could be used to predict the solubility of CO2 in n-decane under different conditions. The solubility of CO2 in n-decane + n-hexane system ranged from 1.0127 mol/kg to 65.7286 mol/kg. It was found that, under low-pressure conditions, the addition of co-solvent n-hexane did not enhance the solubility of CO2, while it had a certain enhancement effect on the dissolution of CO2 under high-pressure conditions. As the temperature increased from 303.15 K to 353.15 K, the enhancement efficiency of the solubility of CO2 also increased from 1.34~2.05% to 8.17~9.82%, and the average enhancement efficiency increased from 1.74% to 9.00%. This study provides more CO2 solubility data for CO2-EOR.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.3390/pr11041137
- https://www.mdpi.com/2227-9717/11/4/1137/pdf?version=1680853454
- OA Status
- gold
- Cited By
- 7
- References
- 40
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4362698847
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4362698847Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.3390/pr11041137Digital Object Identifier
- Title
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Integrated a Fused Silica Capillary Cell and In Situ Raman Spectroscopy for Determining the Solubility of CO2 in n-Decane and n-Decane + n-Hexane SystemWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-04-07Full publication date if available
- Authors
-
Junliang Wang, Zhenzhen Zhang, Quanyuan Wang, Tianhong Lou, Zhiyan Pan, Mian HuList of authors in order
- Landing page
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https://doi.org/10.3390/pr11041137Publisher landing page
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https://www.mdpi.com/2227-9717/11/4/1137/pdf?version=1680853454Direct link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.mdpi.com/2227-9717/11/4/1137/pdf?version=1680853454Direct OA link when available
- Concepts
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Solubility, Decane, Dissolution, Hexane, Solvent, Chemistry, Analytical Chemistry (journal), Hildebrand solubility parameter, Chromatography, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
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7Total citation count in OpenAlex
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2024: 3, 2023: 4Per-year citation counts (last 5 years)
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40Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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| primary_location.landing_page_url | https://doi.org/10.3390/pr11041137 |
| publication_date | 2023-04-07 |
| publication_year | 2023 |
| referenced_works | https://openalex.org/W2567784893, https://openalex.org/W2795904783, https://openalex.org/W3044445723, https://openalex.org/W2156157987, https://openalex.org/W2014376689, https://openalex.org/W2782933733, https://openalex.org/W2485912529, https://openalex.org/W6757876867, https://openalex.org/W2605105641, https://openalex.org/W2891687895, https://openalex.org/W2763598547, https://openalex.org/W2066746795, https://openalex.org/W2756772778, https://openalex.org/W2021129765, https://openalex.org/W1976257237, https://openalex.org/W2333093752, https://openalex.org/W2060285396, https://openalex.org/W2081569072, https://openalex.org/W2071716605, https://openalex.org/W2358237110, https://openalex.org/W2011731363, https://openalex.org/W2920934580, https://openalex.org/W1972921471, https://openalex.org/W2039904122, https://openalex.org/W1967419525, https://openalex.org/W2111699039, https://openalex.org/W2010831738, https://openalex.org/W2074543726, https://openalex.org/W2781537288, https://openalex.org/W2937928560, https://openalex.org/W6793512536, https://openalex.org/W2184593311, https://openalex.org/W2326436929, https://openalex.org/W2068728652, https://openalex.org/W2062942651, https://openalex.org/W1979270578, https://openalex.org/W2148775034, https://openalex.org/W2605080048, https://openalex.org/W2029113665, https://openalex.org/W2911824695 |
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| abstract_inverted_index.A | 51 |
| abstract_inverted_index.K | 28, 31, 199 |
| abstract_inverted_index.a | 23, 41, 181 |
| abstract_inverted_index.15 | 36 |
| abstract_inverted_index.As | 193 |
| abstract_inverted_index.In | 13, 64 |
| abstract_inverted_index.It | 159 |
| abstract_inverted_index.K, | 202 |
| abstract_inverted_index.be | 130 |
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| abstract_inverted_index.of | 3, 18, 70, 76, 96, 136, 145, 168, 176, 188, 206, 209 |
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| abstract_inverted_index.to | 35, 60, 66, 132, 156, 200, 215, 225 |
| abstract_inverted_index.up | 34 |
| abstract_inverted_index.(3% | 83 |
| abstract_inverted_index.CO2 | 4, 19, 53, 71, 77, 97, 137, 146, 189, 210, 231 |
| abstract_inverted_index.MPa | 37 |
| abstract_inverted_index.The | 90, 103, 143 |
| abstract_inverted_index.and | 29, 32, 80, 117, 217 |
| abstract_inverted_index.did | 171 |
| abstract_inverted_index.for | 7, 234 |
| abstract_inverted_index.had | 180 |
| abstract_inverted_index.not | 172 |
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| abstract_inverted_index.the | 1, 16, 61, 68, 74, 94, 106, 114, 118, 126, 134, 166, 174, 186, 194, 203, 207, 218 |
| abstract_inverted_index.was | 38, 57, 86, 100, 122, 160 |
| abstract_inverted_index.wt) | 84 |
| abstract_inverted_index.CO2, | 177 |
| abstract_inverted_index.This | 227 |
| abstract_inverted_index.also | 87, 211 |
| abstract_inverted_index.cell | 45 |
| abstract_inverted_index.data | 104, 233 |
| abstract_inverted_index.from | 105, 153, 197, 213, 223 |
| abstract_inverted_index.good | 111 |
| abstract_inverted_index.mean | 119 |
| abstract_inverted_index.more | 230 |
| abstract_inverted_index.situ | 48 |
| abstract_inverted_index.that | 93, 125 |
| abstract_inverted_index.this | 14 |
| abstract_inverted_index.used | 131 |
| abstract_inverted_index.were | 109 |
| abstract_inverted_index.with | 46, 113 |
| abstract_inverted_index.1.74% | 224 |
| abstract_inverted_index.Raman | 49 |
| abstract_inverted_index.could | 129 |
| abstract_inverted_index.data, | 116 |
| abstract_inverted_index.found | 161 |
| abstract_inverted_index.fused | 42 |
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| abstract_inverted_index.range | 25 |
| abstract_inverted_index.study | 228 |
| abstract_inverted_index.that, | 162 |
| abstract_inverted_index.under | 140, 163, 190 |
| abstract_inverted_index.using | 40 |
| abstract_inverted_index.while | 178 |
| abstract_inverted_index.work, | 15 |
| abstract_inverted_index.1.0127 | 154 |
| abstract_inverted_index.3.65%, | 123 |
| abstract_inverted_index.303.15 | 27, 198 |
| abstract_inverted_index.353.15 | 30, 201 |
| abstract_inverted_index.9.00%. | 226 |
| abstract_inverted_index.effect | 184 |
| abstract_inverted_index.mol/kg | 155 |
| abstract_inverted_index.ranged | 152 |
| abstract_inverted_index.silica | 43 |
| abstract_inverted_index.system | 151 |
| abstract_inverted_index.65.7286 | 157 |
| abstract_inverted_index.average | 219 |
| abstract_inverted_index.between | 26 |
| abstract_inverted_index.certain | 182 |
| abstract_inverted_index.enhance | 173 |
| abstract_inverted_index.improve | 67 |
| abstract_inverted_index.mixture | 85 |
| abstract_inverted_index.mol/kg. | 102, 158 |
| abstract_inverted_index.predict | 133 |
| abstract_inverted_index.results | 91 |
| abstract_inverted_index.CO2-EOR. | 235 |
| abstract_inverted_index.addition | 167 |
| abstract_inverted_index.critical | 6 |
| abstract_inverted_index.measured | 39 |
| abstract_inverted_index.n-decane | 21, 79, 99, 139, 148 |
| abstract_inverted_index.n-hexane | 82, 150, 170 |
| abstract_inverted_index.obtained | 58 |
| abstract_inverted_index.provides | 229 |
| abstract_inverted_index.recovery | 11 |
| abstract_inverted_index.relative | 120 |
| abstract_inverted_index.results. | 63 |
| abstract_inverted_index.according | 59 |
| abstract_inverted_index.agreement | 112 |
| abstract_inverted_index.capillary | 44 |
| abstract_inverted_index.deviation | 121 |
| abstract_inverted_index.different | 141 |
| abstract_inverted_index.increased | 196, 212, 222 |
| abstract_inverted_index.indicated | 92 |
| abstract_inverted_index.n-decane, | 73 |
| abstract_inverted_index.pressures | 33 |
| abstract_inverted_index.(CO2-EOR). | 12 |
| abstract_inverted_index.1.34~2.05% | 214 |
| abstract_inverted_index.co-solvent | 81, 169 |
| abstract_inverted_index.efficiency | 205, 221 |
| abstract_inverted_index.indicating | 124 |
| abstract_inverted_index.prediction | 55, 107, 127 |
| abstract_inverted_index.solubility | 2, 17, 54, 69, 75, 95, 135, 144, 175, 208, 232 |
| abstract_inverted_index.8.17~9.82%, | 216 |
| abstract_inverted_index.conditions, | 165 |
| abstract_inverted_index.conditions. | 142, 192 |
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| abstract_inverted_index.enhancement | 183, 204, 220 |
| abstract_inverted_index.temperature | 24, 195 |
| abstract_inverted_index.CO2-enhanced | 9 |
| abstract_inverted_index.experimental | 62, 115 |
| abstract_inverted_index.implementing | 8 |
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| abstract_inverted_index.investigated. | 89 |
| abstract_inverted_index.spectroscopy. | 50 |
| abstract_inverted_index.1.6355~64.0084 | 101 |
| abstract_inverted_index.semi-empirical | 52 |
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| cited_by_percentile_year.min | 96 |
| corresponding_author_ids | https://openalex.org/A5076937456 |
| countries_distinct_count | 1 |
| institutions_distinct_count | 6 |
| corresponding_institution_ids | https://openalex.org/I55712492 |
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| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |